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Opt Lett. 1996 Aug 15;21(16):1286-8. doi: 10.1364/ol.21.001286.

High-precision intensity-selective observation of multiphoton ionization: a new method of photoelectron spectroscopy.

Optics letters

P Hansch, L D Van Woerkom

PMID: 19876327 DOI: 10.1364/ol.21.001286

Abstract

We have developed a novel method of time-of-f light (TOF) photoelectron spectroscopy that permits observation of multiphoton ionizations with extremely high precision, especially for low-probability events. By scanning the laser-produced ionization region across a pinhole we can select specific laser peak intensities. The volumes occupied by low intensities rise rapidly compared with traditional straight TOF spectroscopy, resulting in high signal gains. This technique presents a new way of observing fundamental laser-matter interactions.

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