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Phys Rev Lett. 2010 Jan 22;104(3):037203. doi: 10.1103/PhysRevLett.104.037203. Epub 2010 Jan 21.

Entanglement in supramolecular spin systems of two weakly coupled antiferromagnetic rings (purple-Cr7Ni).

Physical review letters

A Candini, G Lorusso, F Troiani, A Ghirri, S Carretta, P Santini, G Amoretti, C Muryn, F Tuna, G Timco, E J L McInnes, R E P Winpenny, W Wernsdorfer, M Affronte

Affiliations

  1. National Research Center on nanoStructures and bioSystems at Surfaces (S3), CNR-INFM, 41100 Modena, Italy.

PMID: 20366678 DOI: 10.1103/PhysRevLett.104.037203

Abstract

We characterize supramolecular magnetic structures, consisting of two weakly coupled antiferromagnetic rings, by low-temperature specific heat, susceptibility, magnetization and electron paramagnetic resonance measurements. Intra- and inter-ring interactions are modeled through a microscopic spin-Hamiltonian approach that reproduces all the experimental data quantitatively and legitimates the use of an effective two-qubit picture. Spin entanglement between the rings is experimentally demonstrated through magnetic susceptibility below 50 mK and theoretically quantified by the concurrence.

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