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Phys Rev Lett. 2014 Aug 08;113(6):067203. doi: 10.1103/PhysRevLett.113.067203. Epub 2014 Aug 06.

Oscillations of the orbital magnetic moment due to d-band quantum well states.

Physical review letters

M Dąbrowski, T R F Peixoto, M Pazgan, A Winkelmann, M Cinal, T Nakagawa, Y Takagi, T Yokoyama, F Bisio, U Bauer, F Yildiz, M Przybylski, J Kirschner

Affiliations

  1. Max-Planck-Institut für Mikrostrukturphysik, 06120 Halle, Germany.
  2. Institute of Physical Chemistry, Polish Academy of Sciences, 01-224 Warsaw, Poland.
  3. Institute for Molecular Science, Myodaiji-cho, Okazaki, Aichi 444-8585, Japan.
  4. CNR-SPIN Corso Perrone 24, I-16152 Genova, Italy.
  5. Max-Planck-Institut für Mikrostrukturphysik, 06120 Halle, Germany and Faculty of Physics and Applied Computer Science, and Academic Centre for Materials and Nanotechnology, AGH University of Science and Technology, 30-059 Kraków, Poland.
  6. Max-Planck-Institut für Mikrostrukturphysik, 06120 Halle, Germany and Naturwissenschaftliche Fakultät II, Martin-Luther-Universität Halle-Wittenberg, 06120 Halle, Germany.

PMID: 25148348 DOI: 10.1103/PhysRevLett.113.067203

Abstract

The effect of electron confinement on the magnetocrystalline anisotropy of ultrathin bcc Fe films is explored by combining photoemission spectroscopy, x-ray magnetic circular dichroism, and magneto-optical Kerr effect measurements. Pronounced thickness-dependent variations in the magnetocrystalline anisotropy are ascribed to periodic changes in the density of states at the Fermi level, induced by quantization of d(xz), d(yz) out-of-plane orbitals. Our results reveal a direct correlation between quantum well states, the orbital magnetic moment, and the magnetocrystalline anisotropy.

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