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Nat Commun. 2015 Jul 03;6:7614. doi: 10.1038/ncomms8614.

Local destruction of superconductivity by non-magnetic impurities in mesoscopic iron-based superconductors.

Nature communications

Jun Li, Min Ji, Tobias Schwarz, Xiaoxing Ke, Gustaaf Van Tendeloo, Jie Yuan, Paulo J Pereira, Ya Huang, Gufei Zhang, Hai-Luke Feng, Ya-Hua Yuan, Takeshi Hatano, Reinhold Kleiner, Dieter Koelle, Liviu F Chibotaru, Kazunari Yamaura, Hua-Bing Wang, Pei-Heng Wu, Eiji Takayama-Muromachi, Johan Vanacken, Victor V Moshchalkov

Affiliations

  1. 1] INPAC-Institute for Nanoscale Physics and Chemistry, KU Leuven, Celestijnenlaan 200D, Leuven B-3001, Belgium [2] Research Institute of Superconductor Electronics, Nanjing University, Nanjing 210093, China [3] National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan.
  2. 1] Research Institute of Superconductor Electronics, Nanjing University, Nanjing 210093, China [2] National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan.
  3. Physikalisches Institut-Experimentalphysik II and Center for Collective Quantum Phenomena in LISA+, Universität Tübingen, Auf der Morgenstelle 14, Tübingen D-72076, Germany.
  4. Electron Microscopy for Materials Research (EMAT), University of Antwerp, Groenenborgerlaan 171, Antwerp B-2020, Belgium.
  5. 1] National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan [2] Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
  6. Division of Quantum and Physical Chemistry and INPAC-Institute for Nanoscale Physics and Chemistry, KU Leuven, Celestijnenlaan 200F, Leuven B-3001, Belgium.
  7. INPAC-Institute for Nanoscale Physics and Chemistry, KU Leuven, Celestijnenlaan 200D, Leuven B-3001, Belgium.
  8. 1] National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan [2] Graduate School of Chemical Science and Engineering, Hokkaido University, Hokkaido 060-0810, Japan.
  9. National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan.
  10. Research Institute of Superconductor Electronics, Nanjing University, Nanjing 210093, China.
  11. 1] Graduate School of Chemical Science and Engineering, Hokkaido University, Hokkaido 060-0810, Japan [2] WPI-MANA, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan.

PMID: 26139568 PMCID: PMC4506518 DOI: 10.1038/ncomms8614

Abstract

The determination of the pairing symmetry is one of the most crucial issues for the iron-based superconductors, for which various scenarios are discussed controversially. Non-magnetic impurity substitution is one of the most promising approaches to address the issue, because the pair-breaking mechanism from the non-magnetic impurities should be different for various models. Previous substitution experiments demonstrated that the non-magnetic zinc can suppress the superconductivity of various iron-based superconductors. Here we demonstrate the local destruction of superconductivity by non-magnetic zinc impurities in Ba0.5K0.5Fe2As2 by exploring phase-slip phenomena in a mesoscopic structure with 119 × 102 nm(2) cross-section. The impurities suppress superconductivity in a three-dimensional 'Swiss cheese'-like pattern with in-plane and out-of-plane characteristic lengths slightly below ∼1.34 nm. This causes the superconducting order parameter to vary along abundant narrow channels with effective cross-section of a few square nanometres. The local destruction of superconductivity can be related to Cooper pair breaking by non-magnetic impurities.

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