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Phys Rev Lett. 2015 Aug 28;115(9):093602. doi: 10.1103/PhysRevLett.115.093602. Epub 2015 Aug 24.

All-Optical Preparation of Coherent Dark States of a Single Rare Earth Ion Spin in a Crystal.

Physical review letters

Kangwei Xia, Roman Kolesov, Ya Wang, Petr Siyushev, Rolf Reuter, Thomas Kornher, Nadezhda Kukharchyk, Andreas D Wieck, Bruno Villa, Sen Yang, Jörg Wrachtrup

Affiliations

  1. 3. Physikalisches Institut, Universität Stuttgart, and Stuttgart Research Center of Photonic Engineering (SCoPE), Pfaffenwaldring 57, D-70569 Stuttgart, Germany.
  2. Institute for Quantum Optics and Center for Integrated Quantum Science and Technology (IQst), Universität Ulm, Universität Ost, Raum N25, D-89081 Ulm, Germany.
  3. Ruhr-Universität Bochum, Universitätsstraße 150 Gebäude NB, D-44780 Bochum, Germany.

PMID: 26371651 DOI: 10.1103/PhysRevLett.115.093602

Abstract

All-optical addressing and coherent control of single solid-state based quantum bits is a key tool for fast and precise control of ground-state spin qubits. So far, all-optical addressing of qubits was demonstrated only in a very few systems, such as color centers and quantum dots. Here, we perform high-resolution spectroscopic of native and implanted single rare earth ions in solid, namely, a cerium ion in yttrium aluminum garnet (YAG) crystal. We find narrow and spectrally stable optical transitions between the spin sublevels of the ground and excited optical states. Utilizing these transitions we demonstrate the generation of a coherent dark state in electron spin sublevels of a single Ce^{3+} ion in YAG by coherent population trapping.

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