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Appl Radiat Isot. 2016 Jan;107:187-190. doi: 10.1016/j.apradiso.2015.10.006. Epub 2015 Oct 08.

³⁹Ar/Ar measurements using ultra-low background proportional counters.

Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine

Jeter Hall, Craig E Aalseth, Ricco M Bonicalzi, Jill M Brandenberger, Anthony R Day, Paul H Humble, Emily K Mace, Mark E Panisko, Allen Seifert

Affiliations

  1. Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99352, United States. Electronic address: [email protected].
  2. Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99352, United States.

PMID: 26516993 DOI: 10.1016/j.apradiso.2015.10.006

Abstract

Age-dating groundwater and seawater using the (39)Ar/Ar ratio is an important tool to understand water mass-flow rates and mean residence time. Low-background proportional counters developed at Pacific Northwest National Laboratory use mixtures of argon and methane as counting gas. We demonstrate sensitivity to (39)Ar by comparing geological (ancient) argon recovered from a carbon dioxide gas well and commercial argon. The demonstrated sensitivity to the (39)Ar/Ar ratio is sufficient to date water masses as old as 1000 years.

Copyright © 2015 Elsevier Ltd. All rights reserved.

Keywords: (39)Ar; Low level couning; Water age-dating

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