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Kimberg V, Sanchez-Gonzalez A, Mercadier L, et al. Stimulated X-ray Raman scattering - a critical assessment of the building block of nonlinear X-ray spectroscopy. Faraday Discuss. 2016;194:305-324doi: 10.1039/c6fd00103c.
Kimberg, V., Sanchez-Gonzalez, A., Mercadier, L., Weninger, C., Lutman, A., Ratner, D., Coffee, R., Bucher, M., Mucke, M., Agåker, M., Såthe, C., Bostedt, C., Nordgren, J., Rubensson, J. E., & Rohringer, N. (2016). Stimulated X-ray Raman scattering - a critical assessment of the building block of nonlinear X-ray spectroscopy. Faraday discussions, 194305-324. https://doi.org/10.1039/c6fd00103c
Kimberg, Victor, et al. "Stimulated X-ray Raman scattering - a critical assessment of the building block of nonlinear X-ray spectroscopy." Faraday discussions vol. 194 (2016): 305-324. doi: https://doi.org/10.1039/c6fd00103c
Kimberg V, Sanchez-Gonzalez A, Mercadier L, Weninger C, Lutman A, Ratner D, Coffee R, Bucher M, Mucke M, Agåker M, Såthe C, Bostedt C, Nordgren J, Rubensson JE, Rohringer N. Stimulated X-ray Raman scattering - a critical assessment of the building block of nonlinear X-ray spectroscopy. Faraday Discuss. 2016 Dec 16;194:305-324. doi: 10.1039/c6fd00103c. PMID: 27711899.
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Faraday Discuss. 2016 Dec 16;194:305-324. doi: 10.1039/c6fd00103c.

Stimulated X-ray Raman scattering - a critical assessment of the building block of nonlinear X-ray spectroscopy.

Faraday discussions

Victor Kimberg, Alvaro Sanchez-Gonzalez, Laurent Mercadier, Clemens Weninger, Alberto Lutman, Daniel Ratner, Ryan Coffee, Maximilian Bucher, Melanie Mucke, Marcus Agåker, Conny Såthe, Christoph Bostedt, Joseph Nordgren, Jan Erik Rubensson, Nina Rohringer

Affiliations

  1. Max Planck Institute for the Structure and Dynamics of Matter, Hamburg, Germany. [email protected] [email protected] and Royal Institute of Technology, Stockholm, Sweden.
  2. Imperial College, Department of Physics, London, UK.
  3. Max Planck Institute for the Structure and Dynamics of Matter, Hamburg, Germany. [email protected] [email protected].
  4. Max Planck Institute for the Structure and Dynamics of Matter, Hamburg, Germany. [email protected] [email protected] and LCLS, SLAC National Accelerator Laboratory, Menlo Park, California, USA.
  5. LCLS, SLAC National Accelerator Laboratory, Menlo Park, California, USA.
  6. LCLS, SLAC National Accelerator Laboratory, Menlo Park, California, USA and Argonne National Laboratory, Illinois, USA.
  7. Department of Physics and Astronomy, Uppsala University, Uppsala, Sweden.
  8. Argonne National Laboratory, Illinois, USA.

PMID: 27711899 DOI: 10.1039/c6fd00103c

Abstract

With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets.

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