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Phys Rev E. 2016 Dec;94(6):062610. doi: 10.1103/PhysRevE.94.062610. Epub 2016 Dec 27.

Discontinuous thinning in active microrheology of soft complex matter.

Physical review. E

R Wulfert, U Seifert, T Speck

Affiliations

  1. II. Institut für Theoretische Physik, Universität Stuttgart, Pfaffenwaldring 57, 70550 Stuttgart, Germany.
  2. Institut für Physik, Johannes Gutenberg-Universität Mainz, Staudingerweg 7-9, 55128 Mainz, Germany.

PMID: 28085442 DOI: 10.1103/PhysRevE.94.062610

Abstract

Employing theory and numerical simulations, we demonstrate discontinuous force thinning due to the driven motion of an external probe in a host medium. We consider two cases: an ideal structureless medium (modeling ultrasoft materials such as polymer melts) and a dilute bath of interacting repulsive particles. When the driving of the probe exceeds a critical force, the microviscosity of the medium drops abruptly by about an order of magnitude. This phenomenon occurs for strong attractive interactions between a large probe and a sufficiently dense host medium.

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