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Cliffe MJ, Castillo-Martínez E, Wu Y, et al. Metal-Organic Nanosheets Formed via Defect-Mediated Transformation of a Hafnium Metal-Organic Framework. J Am Chem Soc. 2017;139(15):5397-5404doi: 10.1021/jacs.7b00106.
Cliffe, M. J., Castillo-Martínez, E., Wu, Y., Lee, J., Forse, A. C., Firth, F. C. N., Moghadam, P. Z., Fairen-Jimenez, D., Gaultois, M. W., Hill, J. A., Magdysyuk, O. V., Slater, B., Goodwin, A. L., & Grey, C. P. (2017). Metal-Organic Nanosheets Formed via Defect-Mediated Transformation of a Hafnium Metal-Organic Framework. Journal of the American Chemical Society, 139(15), 5397-5404. https://doi.org/10.1021/jacs.7b00106
Cliffe, Matthew J, et al. "Metal-Organic Nanosheets Formed via Defect-Mediated Transformation of a Hafnium Metal-Organic Framework." Journal of the American Chemical Society vol. 139,15 (2017): 5397-5404. doi: https://doi.org/10.1021/jacs.7b00106
Cliffe MJ, Castillo-Martínez E, Wu Y, Lee J, Forse AC, Firth FCN, Moghadam PZ, Fairen-Jimenez D, Gaultois MW, Hill JA, Magdysyuk OV, Slater B, Goodwin AL, Grey CP. Metal-Organic Nanosheets Formed via Defect-Mediated Transformation of a Hafnium Metal-Organic Framework. J Am Chem Soc. 2017 Apr 19;139(15):5397-5404. doi: 10.1021/jacs.7b00106. Epub 2017 Apr 05. PMID: 28343394; PMCID: PMC5469521.
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J Am Chem Soc. 2017 Apr 19;139(15):5397-5404. doi: 10.1021/jacs.7b00106. Epub 2017 Apr 05.

Metal-Organic Nanosheets Formed via Defect-Mediated Transformation of a Hafnium Metal-Organic Framework.

Journal of the American Chemical Society

Matthew J Cliffe, Elizabeth Castillo-Martínez, Yue Wu, Jeongjae Lee, Alexander C Forse, Francesca C N Firth, Peyman Z Moghadam, David Fairen-Jimenez, Michael W Gaultois, Joshua A Hill, Oxana V Magdysyuk, Ben Slater, Andrew L Goodwin, Clare P Grey

Affiliations

  1. Department of Chemistry, University of Cambridge , Lensfield Road, Cambridge CB2 1EW, U.K.
  2. Department of Materials Science & Metallurgy, University of Cambridge , 27 Charles Babbage Road, Cambridge CB3 0FS, U.K.
  3. Department of Chemical Engineering and Biotechnology, University of Cambridge , Pembroke Street, Cambridge CB2 3RA, U.K.
  4. Department of Chemistry, University of Oxford , South Parks Road, Oxford OX1 3QR, U.K.
  5. Diamond Light Source Ltd. , Harwell Science and Innovation Campus, Didcot, Oxfordshire OX11 0DE, U.K.
  6. Department of Chemistry, University College London , 20 Gordon Street, London WC1H 0AJ, U.K.

PMID: 28343394 PMCID: PMC5469521 DOI: 10.1021/jacs.7b00106

Abstract

We report a hafnium-containing MOF, hcp UiO-67(Hf), which is a ligand-deficient layered analogue of the face-centered cubic fcu UiO-67(Hf). hcp UiO-67 accommodates its lower ligand:metal ratio compared to fcu UiO-67 through a new structural mechanism: the formation of a condensed "double cluster" (Hf

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