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Jacobson P, Muenks M, Laskin G, et al. Potential energy-driven spin manipulation via a controllable hydrogen ligand. Sci Adv. 2017;3(4):e1602060doi: 10.1126/sciadv.1602060.
Jacobson, P., Muenks, M., Laskin, G., Brovko, O., Stepanyuk, V., Ternes, M., & Kern, K. (2017). Potential energy-driven spin manipulation via a controllable hydrogen ligand. Science advances, 3(4), e1602060. https://doi.org/10.1126/sciadv.1602060
Jacobson, Peter, et al. "Potential energy-driven spin manipulation via a controllable hydrogen ligand." Science advances vol. 3,4 (2017): e1602060. doi: https://doi.org/10.1126/sciadv.1602060
Jacobson P, Muenks M, Laskin G, Brovko O, Stepanyuk V, Ternes M, Kern K. Potential energy-driven spin manipulation via a controllable hydrogen ligand. Sci Adv. 2017 Apr 14;3(4):e1602060. doi: 10.1126/sciadv.1602060. eCollection 2017 Apr. PMID: 28439541; PMCID: PMC5392040.
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Sci Adv. 2017 Apr 14;3(4):e1602060. doi: 10.1126/sciadv.1602060. eCollection 2017 Apr.

Potential energy-driven spin manipulation via a controllable hydrogen ligand.

Science advances

Peter Jacobson, Matthias Muenks, Gennadii Laskin, Oleg Brovko, Valeri Stepanyuk, Markus Ternes, Klaus Kern

Affiliations

  1. Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569 Stuttgart, Germany.
  2. Abdus Salam International Centre for Theoretical Physics, Trieste, Italy.
  3. Max Planck Institute of Microstructure Physics, Weinberg 2, 06120, Halle (Saale), Germany.
  4. Institut de Physique, École Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland.

PMID: 28439541 PMCID: PMC5392040 DOI: 10.1126/sciadv.1602060

Abstract

Spin-bearing molecules can be stabilized on surfaces and in junctions with desirable properties, such as a net spin that can be adjusted by external stimuli. Using scanning probes, initial and final spin states can be deduced from topographic or spectroscopic data, but how the system transitions between these states is largely unknown. We address this question by manipulating the total spin of magnetic cobalt hydride complexes on a corrugated boron nitride surface with a hydrogen-functionalized scanning probe tip by simultaneously tracking force and conductance. When the additional hydrogen ligand is brought close to the cobalt monohydride, switching between a correlated

Keywords: Atomic Force Microscopy; Kondo effect; density functional theory; force spectroscopy; inelastic tunneling; molecular magnetism; nano magnetism; potential energy surfaces; scanning probe microscopy; scanning tunneling spectroscopy

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