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Nano Lett. 2017 Jun 14;17(6):3844-3853. doi: 10.1021/acs.nanolett.7b01253. Epub 2017 May 10.

Role of Nonradiative Defects and Environmental Oxygen on Exciton Recombination Processes in CsPbBr.

Nano letters

Monica Lorenzon, Luca Sortino, Quinten Akkerman, Sara Accornero, Jacopo Pedrini, Mirko Prato, Valerio Pinchetti, Francesco Meinardi, Liberato Manna, Sergio Brovelli

Affiliations

  1. Dipartimento di Scienza dei Materiali, Università degli Studi di Milano-Bicocca , via R. Cozzi 55, 20125 Milano, Italy.

PMID: 28480698 PMCID: PMC6557541 DOI: 10.1021/acs.nanolett.7b01253

Abstract

Lead halide perovskite nanocrystals (NCs) are emerging as optically active materials for solution-processed optoelectronic devices. Despite the technological relevance of tracing rational guidelines for optimizing their performances and stability beyond their intrinsic resilience to structural imperfections, no in-depth study of the role of selective carrier trapping and environmental conditions on their exciton dynamics has been reported to date. Here we conduct spectro-electrochemical (SEC) experiments, side-by-side to oxygen sensing measurements on CsPbBr

Keywords: Perovskite nanocrystals; cesium lead halide perovskites; oxygen sensing; spectro-electrochemistry; surface defects; trapping

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