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Nat Commun. 2017 Jun 09;8:15829. doi: 10.1038/ncomms15829.

Controlling hybrid nonlinearities in transparent conducting oxides via two-colour excitation.

Nature communications

M Clerici, N Kinsey, C DeVault, J Kim, E G Carnemolla, L Caspani, A Shaltout, D Faccio, V Shalaev, A Boltasseva, M Ferrera

Affiliations

  1. School of Engineering, University of Glasgow, Glasgow G12 8LT, UK.
  2. School of Electrical and Computer Engineering and Birck Nanotechnology Center, Purdue University, West Lafayette, Indiana 47907, USA.
  3. Department of Physics &Astronomy and Birck Nanotechnology Center, Purdue University, West Lafayette, Indiana 47907, USA.
  4. Institute of Photonics and Quantum Sciences, Heriot-Watt University, SUPA, Edinburgh, Scotland EH14 4AS, UK.
  5. Institute of Photonics, Department of Physics, University of Strathclyde, Glasgow G1 1RD, UK.

PMID: 28598441 PMCID: PMC5472708 DOI: 10.1038/ncomms15829

Abstract

Nanophotonics and metamaterials have revolutionized the way we think about optical space (ɛ,μ), enabling us to engineer the refractive index almost at will, to confine light to the smallest of the volumes, and to manipulate optical signals with extremely small footprints and energy requirements. Significant efforts are now devoted to finding suitable materials and strategies for the dynamic control of the optical properties. Transparent conductive oxides exhibit large ultrafast nonlinearities under both interband and intraband excitations. Here we show that combining these two effects in aluminium-doped zinc oxide via a two-colour laser field discloses new material functionalities. Owing to the independence of the two nonlinearities, the ultrafast temporal dynamics of the material permittivity can be designed by acting on the amplitude and delay of the two fields. We demonstrate the potential applications of this novel degree of freedom by dynamically addressing the modulation bandwidth and optical spectral tuning of a probe optical pulse.

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