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Phys Chem Chem Phys. 2017 Oct 11;19(39):27007-27014. doi: 10.1039/c7cp04496h.

Transmutation effects on long-term Cs retention in phyllosilicate minerals from first principles.

Physical chemistry chemical physics : PCCP

Michel Sassi, Masahiko Okumura, Masahiko Machida, Kevin M Rosso

Affiliations

  1. Physical Sciences Division, Pacific Northwest National Laboratory, Richland, WA 99354, USA. [email protected].

PMID: 28956574 DOI: 10.1039/c7cp04496h

Abstract

The accidental release and incorporation of radiocesium into soil minerals represents a massive environmental, technical and social challenge. Accurately forecasting the evolving distribution and fate of long- and medium-lived isotopes such as

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