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Carmo Dos Santos NA, Natali M, Badetti E, et al. Cobalt, nickel, and iron complexes of 8-hydroxyquinoline-di(2-picolyl)amine for light-driven hydrogen evolution. Dalton Trans. 2017;46(47):16455-16464doi: 10.1039/c7dt02666h.
Carmo Dos Santos, N. A., Natali, M., Badetti, E., Wurst, K., Licini, G., & Zonta, C. (2017). Cobalt, nickel, and iron complexes of 8-hydroxyquinoline-di(2-picolyl)amine for light-driven hydrogen evolution. Dalton transactions (Cambridge, England : 2003), 46(47), 16455-16464. https://doi.org/10.1039/c7dt02666h
Carmo Dos Santos, Nadia Alessandra, et al. "Cobalt, nickel, and iron complexes of 8-hydroxyquinoline-di(2-picolyl)amine for light-driven hydrogen evolution." Dalton transactions (Cambridge, England : 2003) vol. 46,47 (2017): 16455-16464. doi: https://doi.org/10.1039/c7dt02666h
Carmo Dos Santos NA, Natali M, Badetti E, Wurst K, Licini G, Zonta C. Cobalt, nickel, and iron complexes of 8-hydroxyquinoline-di(2-picolyl)amine for light-driven hydrogen evolution. Dalton Trans. 2017 Dec 21;46(47):16455-16464. doi: 10.1039/c7dt02666h. Epub 2017 Nov 16. PMID: 29143834.
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Dalton Trans. 2017 Dec 21;46(47):16455-16464. doi: 10.1039/c7dt02666h. Epub 2017 Nov 16.

Cobalt, nickel, and iron complexes of 8-hydroxyquinoline-di(2-picolyl)amine for light-driven hydrogen evolution.

Dalton transactions (Cambridge, England : 2003)

Nadia Alessandra Carmo Dos Santos, Mirco Natali, Elena Badetti, Klaus Wurst, Giulia Licini, Cristiano Zonta

Affiliations

  1. Department of Chemical Sciences, University of Padova, Via F. Marzolo 1, 35131 Padova, Italy. [email protected].
  2. Department of Chemical and Pharmaceutical Sciences, University of Ferrara, and Centro Interuniversitario per la Conversione Chimica dell'Energia Solare (SolarChem), sez. di Ferrara, via L. Borsari 46, 44121 Ferrara, Italy. [email protected].
  3. Institute of General, Inorganic and Theoretical Chemistry, University of Innsbruck, A-6020 Innsbruck, Austria.

PMID: 29143834 DOI: 10.1039/c7dt02666h

Abstract

Novel cobalt, nickel, and iron complexes based on the pentadentate 8-hydroxyquinoline-di(2-picolyl)amine ligand were synthesized and thoroughly characterized. X-ray structures of both the cobalt and iron complexes were also obtained, showing the tendency to adopt a pseudo-octahedral geometry by coordination of an additional sixth ligand. These metal complexes were then studied as potential hydrogen-evolving catalysts (HECs) under both electrochemical and light-driven conditions. In particular, two different photochemical systems were tested involving either Ru(bpy)

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