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Phys Rev Lett. 2017 Dec 22;119(25):256404. doi: 10.1103/PhysRevLett.119.256404. Epub 2017 Dec 22.

Dimensionality-Driven Metal-Insulator Transition in Spin-Orbit-Coupled SrIrO_{3}.

Physical review letters

P Schütz, D Di Sante, L Dudy, J Gabel, M Stübinger, M Kamp, Y Huang, M Capone, M-A Husanu, V N Strocov, G Sangiovanni, M Sing, R Claessen

Affiliations

  1. Physikalisches Institut and Röntgen Center for Complex Material Systems (RCCM), Universität Würzburg, Am Hubland, D-97074 Würzburg, Germany.
  2. Institut für Theoretische Physik und Astrophysik, Universität Würzburg, Am Hubland, D-97074 Würzburg, Germany.
  3. Van der Waals-Zeeman Insitute, University of Amsterdam, Science Park 904, 1098 XH Amsterdam, The Netherlands.
  4. CNR-IOM-Democritos National Simulation Centre and International School for Advanced Studies (SISSA), Via Bonomea 265, I-34136 Trieste, Italy.
  5. National Institute of Materials Physics, Atomistilor 405 A, 077125 Magurele, Romania.
  6. Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen, Switzerland.

PMID: 29303315 DOI: 10.1103/PhysRevLett.119.256404

Abstract

Upon reduction of the film thickness we observe a metal-insulator transition in epitaxially stabilized, spin-orbit-coupled SrIrO_{3} ultrathin films. By comparison of the experimental electronic dispersions with density functional theory at various levels of complexity we identify the leading microscopic mechanisms, i.e., a dimensionality-induced readjustment of octahedral rotations, magnetism, and electronic correlations. The astonishing resemblance of the band structure in the two-dimensional limit to that of bulk Sr_{2}IrO_{4} opens new avenues to unconventional superconductivity by "clean" electron doping through electric field gating.

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