Angew Chem Int Ed Engl. 2019 Sep 16;58(38):13400-13404. doi: 10.1002/anie.201908164. Epub 2019 Aug 13.

Atomic/Molecular Layer Deposited Iron-Azobenzene Framework Thin Films for Stimuli-Induced Gas Molecule Capture/Release.

Angewandte Chemie (International ed. in English)

Aida Khayyami, Anish Philip, Maarit Karppinen

PMID: 31318130 DOI: 10.1002/anie.201908164

Abstract

The atomic/molecular layer deposition (ALD/MLD) technique provides an elegant way to grow crystalline metal-azobenzene thin films directly from gaseous precursors; the photoactive azobenzene linkers thus form an integral part of the crystal framework. Reversible water capture/release behavior for these thin films can be triggered through the trans-cis photoisomerization reaction of the azobenzene moieties in the structure. The ALD/MLD approach could open up new horizons for example, for the emerging fields of remotely controlled drug delivery and gas storage.

© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Keywords: atomic layer deposition; azobenzene; metal-organic frameworks; molecular layer deposition; thin films

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Publication Types

• Journal Article

Grant support

• 339478/FP7 Ideas: European Research Council
• 296299/Academy of Finland