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Touil A, Broseta D, Desmedt A. Gas Hydrate Crystallization in Thin Glass Capillaries: Roles of Supercooling and Wettability. Langmuir. 2019;35(38):12569-12581doi: 10.1021/acs.langmuir.9b01146.
Touil, A., Broseta, D., & Desmedt, A. (2019). Gas Hydrate Crystallization in Thin Glass Capillaries: Roles of Supercooling and Wettability. Langmuir : the ACS journal of surfaces and colloids, 35(38), 12569-12581. https://doi.org/10.1021/acs.langmuir.9b01146
Touil, Abdelhafid, et al. "Gas Hydrate Crystallization in Thin Glass Capillaries: Roles of Supercooling and Wettability." Langmuir : the ACS journal of surfaces and colloids vol. 35,38 (2019): 12569-12581. doi: https://doi.org/10.1021/acs.langmuir.9b01146
Touil A, Broseta D, Desmedt A. Gas Hydrate Crystallization in Thin Glass Capillaries: Roles of Supercooling and Wettability. Langmuir. 2019 Sep 24;35(38):12569-12581. doi: 10.1021/acs.langmuir.9b01146. Epub 2019 Sep 10. PMID: 31419142.
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Langmuir. 2019 Sep 24;35(38):12569-12581. doi: 10.1021/acs.langmuir.9b01146. Epub 2019 Sep 10.

Gas Hydrate Crystallization in Thin Glass Capillaries: Roles of Supercooling and Wettability.

Langmuir : the ACS journal of surfaces and colloids

Abdelhafid Touil, Daniel Broseta, Arnaud Desmedt

Affiliations

  1. Laboratoire des Fluides Complexes et de leurs Réservoirs (LFCR), UMR 5150 , Centre National de la Recherche Scientifique (CNRS)/TOTAL/Energy Environment Solutions, Université de Pau et des Pays de l'Adour (E2S UPPA) , 64000 Pau , France.
  2. Direction Centrale de Recherche et Développement , Sonatrach , 35000 Boumerdès , Algeria.
  3. Institut des Sciences Moléculaires (ISM), UMR 5255 , Centre National de la Recherche Scientifique (CNRS), Université de Bordeaux , 33405 Talence , France.

PMID: 31419142 DOI: 10.1021/acs.langmuir.9b01146

Abstract

We designed and implemented an experimental methodology to investigate gas hydrate formation and growth around a water-guest meniscus in a thin glass capillary, thus mimicking pore-scale processes in sediments. The glass capillary acts as a high-pressure optical cell in a range of supercooling conditions from 0.1 °C, i.e., very close to hydrate dissociation conditions, to ∼35 °C, very near the metastability limit. Liquid or gaseous CO

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