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Switching from Reactant to Substrate Engineering in the Selective Synthesis of Graphene Nanoribbons.

The journal of physical chemistry letters

Merino-Díez N, Lobo-Checa J, Nita P, Garcia-Lekue A, Basagni A, Vasseur G, Tiso F, Sedona F, Das PK, Fujii J, Vobornik I, Sambi M, Pascual JI, Ortega JE, de Oteyza DG.
PMID: 29688007
J Phys Chem Lett. 2018 May 17;9(10):2510-2517. doi: 10.1021/acs.jpclett.8b00796. Epub 2018 Apr 27.

The challenge of synthesizing graphene nanoribbons (GNRs) with atomic precision is currently being pursued along a one-way road, based on the synthesis of adequate molecular precursors that react in predefined ways through self-assembly processes. The synthetic options for GNR...

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Merino-Díez N, Lobo-Checa J, Nita P, et al. Switching from Reactant to Substrate Engineering in the Selective Synthesis of Graphene Nanoribbons. J Phys Chem Lett. 2018;9(10):2510-2517doi: 10.1021/acs.jpclett.8b00796.
Merino-Díez, N., Lobo-Checa, J., Nita, P., Garcia-Lekue, A., Basagni, A., Vasseur, G., Tiso, F., Sedona, F., Das, P. K., Fujii, J., Vobornik, I., Sambi, M., Pascual, J. I., Ortega, J. E., & de Oteyza, D. G. (2018). Switching from Reactant to Substrate Engineering in the Selective Synthesis of Graphene Nanoribbons. The journal of physical chemistry letters, 9(10), 2510-2517. https://doi.org/10.1021/acs.jpclett.8b00796
Merino-Díez, Néstor, et al. "Switching from Reactant to Substrate Engineering in the Selective Synthesis of Graphene Nanoribbons." The journal of physical chemistry letters vol. 9,10 (2018): 2510-2517. doi: https://doi.org/10.1021/acs.jpclett.8b00796
Merino-Díez N, Lobo-Checa J, Nita P, Garcia-Lekue A, Basagni A, Vasseur G, Tiso F, Sedona F, Das PK, Fujii J, Vobornik I, Sambi M, Pascual JI, Ortega JE, de Oteyza DG. Switching from Reactant to Substrate Engineering in the Selective Synthesis of Graphene Nanoribbons. J Phys Chem Lett. 2018 May 17;9(10):2510-2517. doi: 10.1021/acs.jpclett.8b00796. Epub 2018 Apr 27. PMID: 29688007.
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On-Surface Synthesis of a Five-Membered Carbon Ring from a Terminal Alkynyl Bromide: A [4 + 1] Annulation.

The journal of physical chemistry letters

Wang T, Pan Y, Zhang W, Lawrence J, Mohammed MSG, Huang J, Feng L, Berdonces-Layunta A, Han D, Xu Q, Wu X, Tait SL, de Oteyza DG, Zhu J.
PMID: 32633516
J Phys Chem Lett. 2020 Aug 06;11(15):5902-5907. doi: 10.1021/acs.jpclett.0c01483. Epub 2020 Jul 13.

We report an on-surface synthesis of five-membered carbon ring via a [4 + 1] annulation reaction, starting from a simple terminal alkynyl bromide, 4-(bromoethynyl)biphenyl, on Ag(110). The combination of scanning tunneling microscopy (STM), synchrotron radiation photoemission spectroscopy (SRPES), and...

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Wang T, Pan Y, Zhang W, et al. On-Surface Synthesis of a Five-Membered Carbon Ring from a Terminal Alkynyl Bromide: A [4 + 1] Annulation. J Phys Chem Lett. 2020;11(15):5902-5907doi: 10.1021/acs.jpclett.0c01483.
Wang, T., Pan, Y., Zhang, W., Lawrence, J., Mohammed, M. S. G., Huang, J., Feng, L., Berdonces-Layunta, A., Han, D., Xu, Q., Wu, X., Tait, S. L., de Oteyza, D. G., & Zhu, J. (2020). On-Surface Synthesis of a Five-Membered Carbon Ring from a Terminal Alkynyl Bromide: A [4 + 1] Annulation. The journal of physical chemistry letters, 11(15), 5902-5907. https://doi.org/10.1021/acs.jpclett.0c01483
Wang, Tao, et al. "On-Surface Synthesis of a Five-Membered Carbon Ring from a Terminal Alkynyl Bromide: A [4 + 1] Annulation." The journal of physical chemistry letters vol. 11,15 (2020): 5902-5907. doi: https://doi.org/10.1021/acs.jpclett.0c01483
Wang T, Pan Y, Zhang W, Lawrence J, Mohammed MSG, Huang J, Feng L, Berdonces-Layunta A, Han D, Xu Q, Wu X, Tait SL, de Oteyza DG, Zhu J. On-Surface Synthesis of a Five-Membered Carbon Ring from a Terminal Alkynyl Bromide: A [4 + 1] Annulation. J Phys Chem Lett. 2020 Aug 06;11(15):5902-5907. doi: 10.1021/acs.jpclett.0c01483. Epub 2020 Jul 13. PMID: 32633516.
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Degradation of Soil Humic Extract by Wood- and Soil-Associated Fungi, Bacteria, and Commercial Enzymes.

Microbial ecology

Gramss G, Sorge S, Ziegenhagen D.
PMID: 9929402
Microb Ecol. 1999 Feb;37(2):140-151. doi: 10.1007/s002489900138.

> Abstract An alkaline humic extract (HE) of a black calcareous forest mull was exposed to 36 fungal and 9 eubacterial isolates in liquid standing culture. At 21 d in fungi, and 4 d in bacteria, the groups of...

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Gramss G, Sorge S, Ziegenhagen D. Degradation of Soil Humic Extract by Wood- and Soil-Associated Fungi, Bacteria, and Commercial Enzymes. Microb Ecol. 1999;37(2):140-151doi: 10.1007/s002489900138.
Gramss, G., Sorge, S., & Ziegenhagen, D. (1999). Degradation of Soil Humic Extract by Wood- and Soil-Associated Fungi, Bacteria, and Commercial Enzymes. Microbial ecology, 37(2), 140-151. https://doi.org/10.1007/s002489900138
Gramss, et al. "Degradation of Soil Humic Extract by Wood- and Soil-Associated Fungi, Bacteria, and Commercial Enzymes." Microbial ecology vol. 37,2 (1999): 140-151. doi: https://doi.org/10.1007/s002489900138
Gramss G, Sorge S, Ziegenhagen D. Degradation of Soil Humic Extract by Wood- and Soil-Associated Fungi, Bacteria, and Commercial Enzymes. Microb Ecol. 1999 Feb;37(2):140-151. doi: 10.1007/s002489900138. PMID: 9929402.
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Total photoabsorption cross sections for 1H, 2H, and 3He from 200 to 800 MeV.

Physical review. C, Nuclear physics

Ahrens J, Altieri S, Annand JR, Audit G, Beck R, Braghieri A, Crawford RA, d'Hose N, Dolbilkin B, Ghedira L, Isbert V, Kellie JD, Kerhoas S, MacCormick M, MacGregor IJ, Murphy LY, Pedroni P, Pinelli T, Tamas G, Wallace PA, Zabrodin A.
PMID: 9970910
Phys Rev C Nucl Phys. 1996 Jan;53(1):41-49. doi: 10.1103/physrevc.53.41.

No abstract available.

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Ahrens J, Altieri S, Annand JR, et al. Total photoabsorption cross sections for 1H, 2H, and 3He from 200 to 800 MeV. Phys Rev C Nucl Phys. 1996;53(1):41-49doi: 10.1103/physrevc.53.41.
Ahrens, J., Altieri, S., Annand, J. R., Audit, G., Beck, R., Braghieri, A., Crawford, R. A., d'Hose, N., Dolbilkin, B., Ghedira, L., Isbert, V., Kellie, J. D., Kerhoas, S., MacCormick, M., MacGregor, I. J., Murphy, L. Y., Pedroni, P., Pinelli, T., Tamas, G., Wallace, P. A., & Zabrodin, A. (1996). Total photoabsorption cross sections for 1H, 2H, and 3He from 200 to 800 MeV. Physical review. C, Nuclear physics, 53(1), 41-49. https://doi.org/10.1103/physrevc.53.41
Ahrens, et al. "Total photoabsorption cross sections for 1H, 2H, and 3He from 200 to 800 MeV." Physical review. C, Nuclear physics vol. 53,1 (1996): 41-49. doi: https://doi.org/10.1103/physrevc.53.41
Ahrens J, Altieri S, Annand JR, Audit G, Beck R, Braghieri A, Crawford RA, d'Hose N, Dolbilkin B, Ghedira L, Isbert V, Kellie JD, Kerhoas S, MacCormick M, MacGregor IJ, Murphy LY, Pedroni P, Pinelli T, Tamas G, Wallace PA, Zabrodin A. Total photoabsorption cross sections for 1H, 2H, and 3He from 200 to 800 MeV. Phys Rev C Nucl Phys. 1996 Jan;53(1):41-49. doi: 10.1103/physrevc.53.41. PMID: 9970910.
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Surface adsorption and lubrication properties of plant and dairy proteins: A comparative study.

Food hydrocolloids

Zembyla M, Liamas E, Andablo-Reyes E, Gu K, Krop EM, Kew B, Sarkar A.
PMID: 33536697
Food Hydrocoll. 2021 Feb;111:106364. doi: 10.1016/j.foodhyd.2020.106364.

The aim of this work was to compare the surface adsorption and lubrication properties of plant and dairy proteins. Whey protein isolate (WPI) and pea protein isolate (PPI) were chosen as model animal and plant proteins, respectively, and various...

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Zembyla M, Liamas E, Andablo-Reyes E, et al. Surface adsorption and lubrication properties of plant and dairy proteins: A comparative study. Food Hydrocoll. 2021;111:106364doi: 10.1016/j.foodhyd.2020.106364.
Zembyla, M., Liamas, E., Andablo-Reyes, E., Gu, K., Krop, E. M., Kew, B., & Sarkar, A. (2021). Surface adsorption and lubrication properties of plant and dairy proteins: A comparative study. Food hydrocolloids, 111106364. https://doi.org/10.1016/j.foodhyd.2020.106364
Zembyla, Morfo, et al. "Surface adsorption and lubrication properties of plant and dairy proteins: A comparative study." Food hydrocolloids vol. 111 (2021): 106364. doi: https://doi.org/10.1016/j.foodhyd.2020.106364
Zembyla M, Liamas E, Andablo-Reyes E, Gu K, Krop EM, Kew B, Sarkar A. Surface adsorption and lubrication properties of plant and dairy proteins: A comparative study. Food Hydrocoll. 2021 Feb;111:106364. doi: 10.1016/j.foodhyd.2020.106364. PMID: 33536697; PMCID: PMC7607376.
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Reassessing Alkyne Coupling Reactions While Studying the Electronic Properties of Diverse Pyrene Linkages at Surfaces.

ACS nano

Lawrence J, Mohammed MSG, Rey D, Aguilar-Galindo F, Berdonces-Layunta A, Peña D, de Oteyza DG.
PMID: 33630588
ACS Nano. 2021 Mar 23;15(3):4937-4946. doi: 10.1021/acsnano.0c09756. Epub 2021 Feb 25.

The combination of alkyne and halogen functional groups in the same molecule allows for the possibility of many different reactions when utilized in on-surface synthesis. Here, we use a pyrene-based precursor with both functionalities to examine the preferential reaction...

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Lawrence J, Mohammed MSG, Rey D, et al. Reassessing Alkyne Coupling Reactions While Studying the Electronic Properties of Diverse Pyrene Linkages at Surfaces. ACS Nano. 2021;15(3):4937-4946doi: 10.1021/acsnano.0c09756.
Lawrence, J., Mohammed, M. S. G., Rey, D., Aguilar-Galindo, F., Berdonces-Layunta, A., Peña, D., & de Oteyza, D. G. (2021). Reassessing Alkyne Coupling Reactions While Studying the Electronic Properties of Diverse Pyrene Linkages at Surfaces. ACS nano, 15(3), 4937-4946. https://doi.org/10.1021/acsnano.0c09756
Lawrence, James, et al. "Reassessing Alkyne Coupling Reactions While Studying the Electronic Properties of Diverse Pyrene Linkages at Surfaces." ACS nano vol. 15,3 (2021): 4937-4946. doi: https://doi.org/10.1021/acsnano.0c09756
Lawrence J, Mohammed MSG, Rey D, Aguilar-Galindo F, Berdonces-Layunta A, Peña D, de Oteyza DG. Reassessing Alkyne Coupling Reactions While Studying the Electronic Properties of Diverse Pyrene Linkages at Surfaces. ACS Nano. 2021 Mar 23;15(3):4937-4946. doi: 10.1021/acsnano.0c09756. Epub 2021 Feb 25. PMID: 33630588; PMCID: PMC7992190.
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Single Photon Emission from a Plasmonic Light Source Driven by a Local Field-Induced Coulomb Blockade.

ACS nano

Leon CC, Gunnarsson O, de Oteyza DG, Rosławska A, Merino P, Grewal A, Kuhnke K, Kern K.
PMID: 32159937
ACS Nano. 2020 Apr 28;14(4):4216-4223. doi: 10.1021/acsnano.9b09299. Epub 2020 Mar 18.

A hallmark of quantum control is the ability to manipulate quantum emission at the nanoscale. Through scanning tunneling microscopy-induced luminescence (STML), we are able to generate plasmonic light originating from inelastic tunneling processes that occur in the vacuum between...

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Leon CC, Gunnarsson O, de Oteyza DG, et al. Single Photon Emission from a Plasmonic Light Source Driven by a Local Field-Induced Coulomb Blockade. ACS Nano. 2020;14(4):4216-4223doi: 10.1021/acsnano.9b09299.
Leon, C. C., Gunnarsson, O., de Oteyza, D. G., Rosławska, A., Merino, P., Grewal, A., Kuhnke, K., & Kern, K. (2020). Single Photon Emission from a Plasmonic Light Source Driven by a Local Field-Induced Coulomb Blockade. ACS nano, 14(4), 4216-4223. https://doi.org/10.1021/acsnano.9b09299
Leon, Christopher C, et al. "Single Photon Emission from a Plasmonic Light Source Driven by a Local Field-Induced Coulomb Blockade." ACS nano vol. 14,4 (2020): 4216-4223. doi: https://doi.org/10.1021/acsnano.9b09299
Leon CC, Gunnarsson O, de Oteyza DG, Rosławska A, Merino P, Grewal A, Kuhnke K, Kern K. Single Photon Emission from a Plasmonic Light Source Driven by a Local Field-Induced Coulomb Blockade. ACS Nano. 2020 Apr 28;14(4):4216-4223. doi: 10.1021/acsnano.9b09299. Epub 2020 Mar 18. PMID: 32159937; PMCID: PMC7199210.
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Ectopic pregnancy in noncommunicating horn of unicornuate uterus: 3D-ultrasound and primary laparoscopic management.

Clinical case reports

Dhanawat J, Pape J, Stuhlmann-Laeisz C, Maass N, Freytag D, Gitas G, Alkatout I.
PMID: 34084520
Clin Case Rep. 2021 May 24;9(5):e04261. doi: 10.1002/ccr3.4261. eCollection 2021 May.

Unicornuate uterus with pregnancy in the noncommunicating rudimentary horn is extremely rare. Diagnosis requires awareness, high suspicion index, 3D ultrasound, and MRI. If missed, it can be catastrophic. Treatment varies across literature. We present a case where detection was...

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Dhanawat J, Pape J, Stuhlmann-Laeisz C, et al. Ectopic pregnancy in noncommunicating horn of unicornuate uterus: 3D-ultrasound and primary laparoscopic management. Clin Case Rep. 2021;9(5):e04261doi: 10.1002/ccr3.4261.
Dhanawat, J., Pape, J., Stuhlmann-Laeisz, C., Maass, N., Freytag, D., Gitas, G., & Alkatout, I. (2021). Ectopic pregnancy in noncommunicating horn of unicornuate uterus: 3D-ultrasound and primary laparoscopic management. Clinical case reports, 9(5), e04261. https://doi.org/10.1002/ccr3.4261
Dhanawat, Juhi, et al. "Ectopic pregnancy in noncommunicating horn of unicornuate uterus: 3D-ultrasound and primary laparoscopic management." Clinical case reports vol. 9,5 (2021): e04261. doi: https://doi.org/10.1002/ccr3.4261
Dhanawat J, Pape J, Stuhlmann-Laeisz C, Maass N, Freytag D, Gitas G, Alkatout I. Ectopic pregnancy in noncommunicating horn of unicornuate uterus: 3D-ultrasound and primary laparoscopic management. Clin Case Rep. 2021 May 24;9(5):e04261. doi: 10.1002/ccr3.4261. eCollection 2021 May. PMID: 34084520; PMCID: PMC8142796.
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The Development of Laparoscopy-A Historical Overview.

Frontiers in surgery

Alkatout I, Mechler U, Mettler L, Pape J, Maass N, Biebl M, Gitas G, Laganà AS, Freytag D.
PMID: 34977146
Front Surg. 2021 Dec 15;8:799442. doi: 10.3389/fsurg.2021.799442. eCollection 2021.

The advent of laparoscopy marked a fundamental change in the evolution of medicine. The procedure progressed consistently after the first time it was performed in a human being nearly a hundred years ago. The 1960's and 1980's witnessed groundbreaking...

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Alkatout I, Mechler U, Mettler L, et al. The Development of Laparoscopy-A Historical Overview. Front Surg. 2021;8:799442doi: 10.3389/fsurg.2021.799442.
Alkatout, I., Mechler, U., Mettler, L., Pape, J., Maass, N., Biebl, M., Gitas, G., Laganà, A. S., & Freytag, D. (2021). The Development of Laparoscopy-A Historical Overview. Frontiers in surgery, 8799442. https://doi.org/10.3389/fsurg.2021.799442
Alkatout, Ibrahim, et al. "The Development of Laparoscopy-A Historical Overview." Frontiers in surgery vol. 8 (2021): 799442. doi: https://doi.org/10.3389/fsurg.2021.799442
Alkatout I, Mechler U, Mettler L, Pape J, Maass N, Biebl M, Gitas G, Laganà AS, Freytag D. The Development of Laparoscopy-A Historical Overview. Front Surg. 2021 Dec 15;8:799442. doi: 10.3389/fsurg.2021.799442. eCollection 2021. PMID: 34977146; PMCID: PMC8714650.
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Chemisorption-Induced Formation of Biphenylene Dimer on Ag(111).

Journal of the American Chemical Society

Zeng Z, Guo D, Wang T, Chen Q, Matěj A, Huang J, Han D, Xu Q, Zhao A, Jelínek P, de Oteyza DG, McEwen JS, Zhu J.
PMID: 34964646
J Am Chem Soc. 2021 Dec 29; doi: 10.1021/jacs.1c08284. Epub 2021 Dec 29.

We report an example that demonstrates the clear interdependence between surface-supported reactions and molecular-adsorption configurations. Two biphenyl-based molecules with two and four bromine substituents, i.e., 2,2'-dibromobiphenyl (DBBP) and 2,2',6,6'-tetrabromo-1,1'-biphenyl (TBBP), show completely different reaction pathways on a Ag(111) surface,...

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Zeng Z, Guo D, Wang T, et al. Chemisorption-Induced Formation of Biphenylene Dimer on Ag(111). J Am Chem Soc. 2021;doi: 10.1021/jacs.1c08284.
Zeng, Z., Guo, D., Wang, T., Chen, Q., Matěj, A., Huang, J., Han, D., Xu, Q., Zhao, A., Jelínek, P., de Oteyza, D. G., McEwen, J. S., & Zhu, J. (2021). Chemisorption-Induced Formation of Biphenylene Dimer on Ag(111). Journal of the American Chemical Society, . https://doi.org/10.1021/jacs.1c08284
Zeng, Zhiwen, et al. "Chemisorption-Induced Formation of Biphenylene Dimer on Ag(111)." Journal of the American Chemical Society vol. (2021). doi: https://doi.org/10.1021/jacs.1c08284
Zeng Z, Guo D, Wang T, Chen Q, Matěj A, Huang J, Han D, Xu Q, Zhao A, Jelínek P, de Oteyza DG, McEwen JS, Zhu J. Chemisorption-Induced Formation of Biphenylene Dimer on Ag(111). J Am Chem Soc. 2021 Dec 29; doi: 10.1021/jacs.1c08284. Epub 2021 Dec 29. PMID: 34964646.
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In Silico Identification of Chikungunya Virus B- and T-Cell Epitopes with High Antigenic Potential for Vaccine Development.

Viruses

Sánchez-Burgos GG, Montalvo-Marin NM, Díaz-Rosado ER, Pérez-Rueda E.
PMID: 34960629
Viruses. 2021 Nov 24;13(12). doi: 10.3390/v13122360.

Reverse vaccinology is an outstanding strategy to identify antigens with high potential for vaccine development. Different parameters of five prediction programs were used to assess their sensitivity and specificity to identify B-cell epitopes of Chikungunya virus (CHIKV) strains reported...

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Sánchez-Burgos GG, Montalvo-Marin NM, Díaz-Rosado ER, et al. In Silico Identification of Chikungunya Virus B- and T-Cell Epitopes with High Antigenic Potential for Vaccine Development. Viruses. 2021;13(12)doi: 10.3390/v13122360.
Sánchez-Burgos, G. G., Montalvo-Marin, N. M., Díaz-Rosado, E. R., & Pérez-Rueda, E. (2021). In Silico Identification of Chikungunya Virus B- and T-Cell Epitopes with High Antigenic Potential for Vaccine Development. Viruses, 13(12), . https://doi.org/10.3390/v13122360
Sánchez-Burgos, Gilma G, et al. "In Silico Identification of Chikungunya Virus B- and T-Cell Epitopes with High Antigenic Potential for Vaccine Development." Viruses vol. 13,12 (2021). doi: https://doi.org/10.3390/v13122360
Sánchez-Burgos GG, Montalvo-Marin NM, Díaz-Rosado ER, Pérez-Rueda E. In Silico Identification of Chikungunya Virus B- and T-Cell Epitopes with High Antigenic Potential for Vaccine Development. Viruses. 2021 Nov 24;13(12). doi: 10.3390/v13122360. PMID: 34960629; PMCID: PMC8706625.
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Challenges in the synthesis of corannulene-based non-planar nanographenes on Au(111) surfaces.

Physical chemistry chemical physics : PCCP

Wang T, Lawrence J, Sumi N, Robles R, Castro-Esteban J, Rey D, Mohammed MSG, Berdonces-Layunta A, Lorente N, Pérez D, Peña D, Corso M, de Oteyza DG.
PMID: 33908516
Phys Chem Chem Phys. 2021 May 12;23(18):10845-10851. doi: 10.1039/d1cp01212f.

The on-surface synthesis of non-planar nanographenes is a challenging task. Herein, with the aid of bond-resolving scanning tunneling microscopy (BRSTM) and density functional theory (DFT) calculations, we present a systematic study aiming at the fabrication of corannulene-based nanographenes via...

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Wang T, Lawrence J, Sumi N, et al. Challenges in the synthesis of corannulene-based non-planar nanographenes on Au(111) surfaces. Phys Chem Chem Phys. 2021;23(18):10845-10851doi: 10.1039/d1cp01212f.
Wang, T., Lawrence, J., Sumi, N., Robles, R., Castro-Esteban, J., Rey, D., Mohammed, M. S. G., Berdonces-Layunta, A., Lorente, N., Pérez, D., Peña, D., Corso, M., & de Oteyza, D. G. (2021). Challenges in the synthesis of corannulene-based non-planar nanographenes on Au(111) surfaces. Physical chemistry chemical physics : PCCP, 23(18), 10845-10851. https://doi.org/10.1039/d1cp01212f
Wang, Tao, et al. "Challenges in the synthesis of corannulene-based non-planar nanographenes on Au(111) surfaces." Physical chemistry chemical physics : PCCP vol. 23,18 (2021): 10845-10851. doi: https://doi.org/10.1039/d1cp01212f
Wang T, Lawrence J, Sumi N, Robles R, Castro-Esteban J, Rey D, Mohammed MSG, Berdonces-Layunta A, Lorente N, Pérez D, Peña D, Corso M, de Oteyza DG. Challenges in the synthesis of corannulene-based non-planar nanographenes on Au(111) surfaces. Phys Chem Chem Phys. 2021 May 12;23(18):10845-10851. doi: 10.1039/d1cp01212f. PMID: 33908516.
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