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Unusual (Z)-selective palladium(II)-catalysed addition of aryl boronic acids to vinylaziridines.

Organic & biomolecular chemistry

Yin J, Mekelburg T, Hyland C.
PMID: 25317543
Org Biomol Chem. 2014 Dec 07;12(45):9113-5. doi: 10.1039/c4ob01786b.

The palladium(II)-catalysed addition of arylboronic acids to vinylaziridines has been developed. This reaction proceeds via an insertion/ring-opening process to provide (Z)-allylsulfonamides preferentially. This stereoselectivity is complimentary to existing methods that typically proceed via a SN2' mechanism to yield (E)-allylsulfonamides....

Cite
Yin J, Mekelburg T, Hyland C. Unusual (Z)-selective palladium(II)-catalysed addition of aryl boronic acids to vinylaziridines. Org Biomol Chem. 2014;12(45):9113-5doi: 10.1039/c4ob01786b.
Yin, J., Mekelburg, T., & Hyland, C. (2014). Unusual (Z)-selective palladium(II)-catalysed addition of aryl boronic acids to vinylaziridines. Organic & biomolecular chemistry, 12(45), 9113-5. https://doi.org/10.1039/c4ob01786b
Yin, JieXiang, et al. "Unusual (Z)-selective palladium(II)-catalysed addition of aryl boronic acids to vinylaziridines." Organic & biomolecular chemistry vol. 12,45 (2014): 9113-5. doi: https://doi.org/10.1039/c4ob01786b
Yin J, Mekelburg T, Hyland C. Unusual (Z)-selective palladium(II)-catalysed addition of aryl boronic acids to vinylaziridines. Org Biomol Chem. 2014 Dec 07;12(45):9113-5. doi: 10.1039/c4ob01786b. PMID: 25317543.
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A Spherically Shielded Triphenylamine and Its Persistent Radical Cation.

Chemistry (Weinheim an der Bergstrasse, Germany)

Schaub TA, Mekelburg T, Dral PO, Miehlich M, Hampel F, Meyer K, Kivala M.
PMID: 31970834
Chemistry. 2020 Mar 12;26(15):3264-3269. doi: 10.1002/chem.202000355. Epub 2020 Feb 21.

This work reports the design and synthesis of a sterically protected triphenylamine scaffold which undergoes one-electron oxidation to form an amine-centered radical cation of remarkable stability. Several structural adjustments were made to tame the inherent reactivity of the radical...

Cite
Schaub TA, Mekelburg T, Dral PO, et al. A Spherically Shielded Triphenylamine and Its Persistent Radical Cation. Chemistry. 2020;26(15):3264-3269doi: 10.1002/chem.202000355.
Schaub, T. A., Mekelburg, T., Dral, P. O., Miehlich, M., Hampel, F., Meyer, K., & Kivala, M. (2020). A Spherically Shielded Triphenylamine and Its Persistent Radical Cation. Chemistry (Weinheim an der Bergstrasse, Germany), 26(15), 3264-3269. https://doi.org/10.1002/chem.202000355
Schaub, Tobias A, et al. "A Spherically Shielded Triphenylamine and Its Persistent Radical Cation." Chemistry (Weinheim an der Bergstrasse, Germany) vol. 26,15 (2020): 3264-3269. doi: https://doi.org/10.1002/chem.202000355
Schaub TA, Mekelburg T, Dral PO, Miehlich M, Hampel F, Meyer K, Kivala M. A Spherically Shielded Triphenylamine and Its Persistent Radical Cation. Chemistry. 2020 Mar 12;26(15):3264-3269. doi: 10.1002/chem.202000355. Epub 2020 Feb 21. PMID: 31970834; PMCID: PMC7154785.
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