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Highly Dispersed SiO(x)/Al2O3 Catalysts Illuminate the Reactivity of Isolated Silanol Sites.

Angewandte Chemie (International ed. in English)

Mouat AR, George C, Kobayashi T, Pruski M, van Duyne RP, Marks TJ, Stair PC.
PMID: 26398359
Angew Chem Int Ed Engl. 2015 Nov 02;54(45):13346-51. doi: 10.1002/anie.201505452. Epub 2015 Sep 23.

The reaction of γ-alumina with tetraethylorthosilicate (TEOS) vapor at low temperatures selectively yields monomeric SiO(x) species on the alumina surface. These isolated (-AlO)3Si(OH) sites are characterized by PXRD, XPS, DRIFTS of adsorbed NH3, CO, and pyridine, and (29)Si and...

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Mouat AR, George C, Kobayashi T, et al. Highly Dispersed SiO(x)/Al2O3 Catalysts Illuminate the Reactivity of Isolated Silanol Sites. Angew Chem Int Ed Engl. 2015;54(45):13346-51doi: 10.1002/anie.201505452.
Mouat, A. R., George, C., Kobayashi, T., Pruski, M., van Duyne, R. P., Marks, T. J., & Stair, P. C. (2015). Highly Dispersed SiO(x)/Al2O3 Catalysts Illuminate the Reactivity of Isolated Silanol Sites. Angewandte Chemie (International ed. in English), 54(45), 13346-51. https://doi.org/10.1002/anie.201505452
Mouat, Aidan R, et al. "Highly Dispersed SiO(x)/Al2O3 Catalysts Illuminate the Reactivity of Isolated Silanol Sites." Angewandte Chemie (International ed. in English) vol. 54,45 (2015): 13346-51. doi: https://doi.org/10.1002/anie.201505452
Mouat AR, George C, Kobayashi T, Pruski M, van Duyne RP, Marks TJ, Stair PC. Highly Dispersed SiO(x)/Al2O3 Catalysts Illuminate the Reactivity of Isolated Silanol Sites. Angew Chem Int Ed Engl. 2015 Nov 02;54(45):13346-51. doi: 10.1002/anie.201505452. Epub 2015 Sep 23. PMID: 26398359.
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Poster 339 Better Outcome Though Devastating Course: A Case Report.

PM & R : the journal of injury, function, and rehabilitation

Pruski A, Shin R, Qu X.
PMID: 27673093
PM R. 2016 Sep;8(9):S271. doi: 10.1016/j.pmrj.2016.07.508. Epub 2016 Sep 24.

No abstract available.

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Pruski A, Shin R, Qu X. Poster 339 Better Outcome Though Devastating Course: A Case Report. PM R. 2016;8(9):S271doi: 10.1016/j.pmrj.2016.07.508.
Pruski, A., Shin, R., & Qu, X. (2016). Poster 339 Better Outcome Though Devastating Course: A Case Report. PM & R : the journal of injury, function, and rehabilitation, 8(9), S271. https://doi.org/10.1016/j.pmrj.2016.07.508
Pruski, April, et al. "Poster 339 Better Outcome Though Devastating Course: A Case Report." PM & R : the journal of injury, function, and rehabilitation vol. 8,9 (2016): S271. doi: https://doi.org/10.1016/j.pmrj.2016.07.508
Pruski A, Shin R, Qu X. Poster 339 Better Outcome Though Devastating Course: A Case Report. PM R. 2016 Sep;8(9):S271. doi: 10.1016/j.pmrj.2016.07.508. Epub 2016 Sep 24. PMID: 27673093.
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In Silico Design of DNP Polarizing Agents: Can Current Dinitroxides Be Improved?.

Chemphyschem : a European journal of chemical physics and physical chemistry

Perras FA, Sadow A, Pruski M.
PMID: 28599086
Chemphyschem. 2017 Aug 18;18(16):2279-2287. doi: 10.1002/cphc.201700299. Epub 2017 Jul 07.

Numerical calculations of enhancement factors offered by dynamic nuclear polarization in solids under magic angle spinning (DNP-MAS) were performed to determine the optimal EPR parameters for a dinitroxide polarizing agent. We found that the DNP performance of a biradical...

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Perras FA, Sadow A, Pruski M. In Silico Design of DNP Polarizing Agents: Can Current Dinitroxides Be Improved?. Chemphyschem. 2017;18(16):2279-2287doi: 10.1002/cphc.201700299.
Perras, F. A., Sadow, A., & Pruski, M. (2017). In Silico Design of DNP Polarizing Agents: Can Current Dinitroxides Be Improved?. Chemphyschem : a European journal of chemical physics and physical chemistry, 18(16), 2279-2287. https://doi.org/10.1002/cphc.201700299
Perras, Frédéric A, et al. "In Silico Design of DNP Polarizing Agents: Can Current Dinitroxides Be Improved?." Chemphyschem : a European journal of chemical physics and physical chemistry vol. 18,16 (2017): 2279-2287. doi: https://doi.org/10.1002/cphc.201700299
Perras FA, Sadow A, Pruski M. In Silico Design of DNP Polarizing Agents: Can Current Dinitroxides Be Improved?. Chemphyschem. 2017 Aug 18;18(16):2279-2287. doi: 10.1002/cphc.201700299. Epub 2017 Jul 07. PMID: 28599086.
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Disturbance Increases Microbial Community Diversity and Production in Marine Sediments.

Frontiers in microbiology

Galand PE, Lucas S, Fagervold SK, Peru E, Pruski AM, Vétion G, Dupuy C, Guizien K.
PMID: 27994581
Front Microbiol. 2016 Dec 02;7:1950. doi: 10.3389/fmicb.2016.01950. eCollection 2016.

Disturbance strongly impacts patterns of community diversity, yet the shape of the diversity-disturbance relationship remains a matter of debate. The topic has been of interest in theoretical ecology for decades as it has practical implications for the understanding of...

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Galand PE, Lucas S, Fagervold SK, et al. Disturbance Increases Microbial Community Diversity and Production in Marine Sediments. Front Microbiol. 2016;7:1950doi: 10.3389/fmicb.2016.01950.
Galand, P. E., Lucas, S., Fagervold, S. K., Peru, E., Pruski, A. M., Vétion, G., Dupuy, C., & Guizien, K. (2016). Disturbance Increases Microbial Community Diversity and Production in Marine Sediments. Frontiers in microbiology, 71950. https://doi.org/10.3389/fmicb.2016.01950
Galand, Pierre E, et al. "Disturbance Increases Microbial Community Diversity and Production in Marine Sediments." Frontiers in microbiology vol. 7 (2016): 1950. doi: https://doi.org/10.3389/fmicb.2016.01950
Galand PE, Lucas S, Fagervold SK, Peru E, Pruski AM, Vétion G, Dupuy C, Guizien K. Disturbance Increases Microbial Community Diversity and Production in Marine Sediments. Front Microbiol. 2016 Dec 02;7:1950. doi: 10.3389/fmicb.2016.01950. eCollection 2016. PMID: 27994581; PMCID: PMC5133735.
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DNP-Enhanced Ultrawideline Solid-State NMR Spectroscopy: Studies of Platinum in Metal-Organic Frameworks.

The journal of physical chemistry letters

Kobayashi T, Perras FA, Goh TW, Metz TL, Huang W, Pruski M.
PMID: 27266444
J Phys Chem Lett. 2016 Jul 07;7(13):2322-7. doi: 10.1021/acs.jpclett.6b00860. Epub 2016 Jun 09.

Ultrawideline dynamic nuclear polarization (DNP)-enhanced (195)Pt solid-state NMR (SSNMR) spectroscopy and theoretical calculations are used to determine the coordination of atomic Pt species supported within the pores of metal-organic frameworks (MOFs). The (195)Pt SSNMR spectra, with breadths reaching 10...

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Kobayashi T, Perras FA, Goh TW, et al. DNP-Enhanced Ultrawideline Solid-State NMR Spectroscopy: Studies of Platinum in Metal-Organic Frameworks. J Phys Chem Lett. 2016;7(13):2322-7doi: 10.1021/acs.jpclett.6b00860.
Kobayashi, T., Perras, F. A., Goh, T. W., Metz, T. L., Huang, W., & Pruski, M. (2016). DNP-Enhanced Ultrawideline Solid-State NMR Spectroscopy: Studies of Platinum in Metal-Organic Frameworks. The journal of physical chemistry letters, 7(13), 2322-7. https://doi.org/10.1021/acs.jpclett.6b00860
Kobayashi, Takeshi, et al. "DNP-Enhanced Ultrawideline Solid-State NMR Spectroscopy: Studies of Platinum in Metal-Organic Frameworks." The journal of physical chemistry letters vol. 7,13 (2016): 2322-7. doi: https://doi.org/10.1021/acs.jpclett.6b00860
Kobayashi T, Perras FA, Goh TW, Metz TL, Huang W, Pruski M. DNP-Enhanced Ultrawideline Solid-State NMR Spectroscopy: Studies of Platinum in Metal-Organic Frameworks. J Phys Chem Lett. 2016 Jul 07;7(13):2322-7. doi: 10.1021/acs.jpclett.6b00860. Epub 2016 Jun 09. PMID: 27266444.
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Engineering Biological C-H Functionalization Leads to Allele-Specific Regulation of Histone Demethylases.

Journal of the American Chemical Society

Breski M, Dey D, Obringer S, Sudhamalla B, Islam K.
PMID: 27709909
J Am Chem Soc. 2016 Oct 19;138(41):13505-13508. doi: 10.1021/jacs.6b08653. Epub 2016 Oct 10.

Oxidative C-H hydroxylation of methyl groups, followed by their removal from DNA, RNA, or histones, is an epigenetic process critical to transcriptional reprogramming and cell fate determination. This reaction is catalyzed by Fe(II)-dependent dioxygenases using the essential metabolite 2-ketoglutarate...

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Breski M, Dey D, Obringer S, et al. Engineering Biological C-H Functionalization Leads to Allele-Specific Regulation of Histone Demethylases. J Am Chem Soc. 2016;138(41):13505-13508doi: 10.1021/jacs.6b08653.
Breski, M., Dey, D., Obringer, S., Sudhamalla, B., & Islam, K. (2016). Engineering Biological C-H Functionalization Leads to Allele-Specific Regulation of Histone Demethylases. Journal of the American Chemical Society, 138(41), 13505-13508. https://doi.org/10.1021/jacs.6b08653
Breski, Megan, et al. "Engineering Biological C-H Functionalization Leads to Allele-Specific Regulation of Histone Demethylases." Journal of the American Chemical Society vol. 138,41 (2016): 13505-13508. doi: https://doi.org/10.1021/jacs.6b08653
Breski M, Dey D, Obringer S, Sudhamalla B, Islam K. Engineering Biological C-H Functionalization Leads to Allele-Specific Regulation of Histone Demethylases. J Am Chem Soc. 2016 Oct 19;138(41):13505-13508. doi: 10.1021/jacs.6b08653. Epub 2016 Oct 10. PMID: 27709909.
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Indirectly detected heteronuclear correlation solid-state NMR spectroscopy of naturally abundant 15N nuclei.

Solid state nuclear magnetic resonance

Althaus SM, Mao K, Stringer JA, Kobayashi T, Pruski M.
PMID: 24287060
Solid State Nucl Magn Reson. 2014 Feb-Apr;57:17-21. doi: 10.1016/j.ssnmr.2013.11.001. Epub 2013 Nov 12.

Two-dimensional indirectly detected through-space and through-bond (1)H{(15)N} solid-state NMR experiments utilizing fast magic angle spinning (MAS) and homonuclear multipulse (1)H decoupling are evaluated. Remarkable efficiency of polarization transfer can be achieved at a MAS rate of 40 kHz by...

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Althaus SM, Mao K, Stringer JA, et al. Indirectly detected heteronuclear correlation solid-state NMR spectroscopy of naturally abundant 15N nuclei. Solid State Nucl Magn Reson. 2013;57:17-21doi: 10.1016/j.ssnmr.2013.11.001.
Althaus, S. M., Mao, K., Stringer, J. A., Kobayashi, T., & Pruski, M. (2014). Indirectly detected heteronuclear correlation solid-state NMR spectroscopy of naturally abundant 15N nuclei. Solid state nuclear magnetic resonance, 5717-21. https://doi.org/10.1016/j.ssnmr.2013.11.001
Althaus, Stacey M, et al. "Indirectly detected heteronuclear correlation solid-state NMR spectroscopy of naturally abundant 15N nuclei." Solid state nuclear magnetic resonance vol. 57 (2014): 17-21. doi: https://doi.org/10.1016/j.ssnmr.2013.11.001
Althaus SM, Mao K, Stringer JA, Kobayashi T, Pruski M. Indirectly detected heteronuclear correlation solid-state NMR spectroscopy of naturally abundant 15N nuclei. Solid State Nucl Magn Reson. 2014 Feb-Apr;57:17-21. doi: 10.1016/j.ssnmr.2013.11.001. Epub 2013 Nov 12. PMID: 24287060.
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Oxidative polymerization of 1,4-diethynylbenzene into highly conjugated poly(phenylene butadiynylene) within the channels of surface-functionalized mesoporous silica and alumina materials.

Journal of the American Chemical Society

Lin VS, Radu DR, Han MK, Deng W, Kuroki S, Shanks BH, Pruski M.
PMID: 12148994
J Am Chem Soc. 2002 Aug 07;124(31):9040-1. doi: 10.1021/ja025925o.

A polyalkynylene-based conducting polymer (molecular wire) has been synthesized within the Cu-functionalized mesoporous MCM-41 silica catalyst. Fluorescence and 13C solid-state NMR provided spectroscopic evidence that the synthesis of extended polymeric chains with a high degree of alignment requires homogeneously...

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Lin VS, Radu DR, Han MK, et al. Oxidative polymerization of 1,4-diethynylbenzene into highly conjugated poly(phenylene butadiynylene) within the channels of surface-functionalized mesoporous silica and alumina materials. J Am Chem Soc. 2002;124(31):9040-1doi: 10.1021/ja025925o.
Lin, V. S., Radu, D. R., Han, M. K., Deng, W., Kuroki, S., Shanks, B. H., & Pruski, M. (2002). Oxidative polymerization of 1,4-diethynylbenzene into highly conjugated poly(phenylene butadiynylene) within the channels of surface-functionalized mesoporous silica and alumina materials. Journal of the American Chemical Society, 124(31), 9040-1. https://doi.org/10.1021/ja025925o
Lin, Victor S-Y, et al. "Oxidative polymerization of 1,4-diethynylbenzene into highly conjugated poly(phenylene butadiynylene) within the channels of surface-functionalized mesoporous silica and alumina materials." Journal of the American Chemical Society vol. 124,31 (2002): 9040-1. doi: https://doi.org/10.1021/ja025925o
Lin VS, Radu DR, Han MK, Deng W, Kuroki S, Shanks BH, Pruski M. Oxidative polymerization of 1,4-diethynylbenzene into highly conjugated poly(phenylene butadiynylene) within the channels of surface-functionalized mesoporous silica and alumina materials. J Am Chem Soc. 2002 Aug 07;124(31):9040-1. doi: 10.1021/ja025925o. PMID: 12148994.
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Nondemolition measurements of a single quantum spin using Josephson oscillations.

Physical review letters

Bulaevskii L, Hruska M, Shnirman A, Smith D, Makhlin Y.
PMID: 15169182
Phys Rev Lett. 2004 Apr 30;92(17):177001. doi: 10.1103/PhysRevLett.92.177001. Epub 2004 Apr 27.

We consider a single localized spin-1/2 between the singlet superconducting leads of a Josephson junction (e.g., a superconducting STM). For the spin subject to a dc magnetic field B parallel z, we study the spin dynamics and the possibility...

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Bulaevskii L, Hruska M, Shnirman A, et al. Nondemolition measurements of a single quantum spin using Josephson oscillations. Phys Rev Lett. 2004;92(17):177001doi: 10.1103/PhysRevLett.92.177001.
Bulaevskii, L., Hruska, M., Shnirman, A., Smith, D., & Makhlin, Y. (2004). Nondemolition measurements of a single quantum spin using Josephson oscillations. Physical review letters, 92(17), 177001. https://doi.org/10.1103/PhysRevLett.92.177001
Bulaevskii, L, et al. "Nondemolition measurements of a single quantum spin using Josephson oscillations." Physical review letters vol. 92,17 (2004): 177001. doi: https://doi.org/10.1103/PhysRevLett.92.177001
Bulaevskii L, Hruska M, Shnirman A, Smith D, Makhlin Y. Nondemolition measurements of a single quantum spin using Josephson oscillations. Phys Rev Lett. 2004 Apr 30;92(17):177001. doi: 10.1103/PhysRevLett.92.177001. Epub 2004 Apr 27. PMID: 15169182.
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Identification of electron beam vibration sources by separation of magnetic distortion from electric distortion on scanning electron microscope imaging.

Journal of microscopy

Pluska M, Czerwinski A, Ratajczak J, Katcki J, Oskwarek Ł, Rak R.
PMID: 20500389
J Microsc. 2010 Mar;237(3):325-8. doi: 10.1111/j.1365-2818.2009.03252.x.

Different types of distortions in scanning electron microscopy require different methods of their elimination, and therefore influence of these types on particular elements of the SEM system should be known. The proposed method allows for separation of the direct...

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Pluska M, Czerwinski A, Ratajczak J, et al. Identification of electron beam vibration sources by separation of magnetic distortion from electric distortion on scanning electron microscope imaging. J Microsc. 2010;237(3):325-8doi: 10.1111/j.1365-2818.2009.03252.x.
Pluska, M., Czerwinski, A., Ratajczak, J., Katcki, J., Oskwarek, �. �., & Rak, R. (2010). Identification of electron beam vibration sources by separation of magnetic distortion from electric distortion on scanning electron microscope imaging. Journal of microscopy, 237(3), 325-8. https://doi.org/10.1111/j.1365-2818.2009.03252.x
Pluska, M, et al. "Identification of electron beam vibration sources by separation of magnetic distortion from electric distortion on scanning electron microscope imaging." Journal of microscopy vol. 237,3 (2010): 325-8. doi: https://doi.org/10.1111/j.1365-2818.2009.03252.x
Pluska M, Czerwinski A, Ratajczak J, Katcki J, Oskwarek Ł, Rak R. Identification of electron beam vibration sources by separation of magnetic distortion from electric distortion on scanning electron microscope imaging. J Microsc. 2010 Mar;237(3):325-8. doi: 10.1111/j.1365-2818.2009.03252.x. PMID: 20500389.
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Molecular ordering of mixed surfactants in mesoporous silicas: a solid-state NMR study.

Solid state nuclear magnetic resonance

Kobayashi T, Mao K, Wang SG, Lin VS, Pruski M.
PMID: 21392947
Solid State Nucl Magn Reson. 2011 May-Jun;39(3):65-71. doi: 10.1016/j.ssnmr.2011.02.001. Epub 2011 Feb 17.

The use of mixed surfactants in the synthesis of mesoporous silica nanoparticles (MSNs) is of importance in the context of adjusting pore structures, sizes and morphologies. In the present study, the arrangement of molecules in micelles produced from a...

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Kobayashi T, Mao K, Wang SG, et al. Molecular ordering of mixed surfactants in mesoporous silicas: a solid-state NMR study. Solid State Nucl Magn Reson. 2011;39(3):65-71doi: 10.1016/j.ssnmr.2011.02.001.
Kobayashi, T., Mao, K., Wang, S. G., Lin, V. S., & Pruski, M. (2011). Molecular ordering of mixed surfactants in mesoporous silicas: a solid-state NMR study. Solid state nuclear magnetic resonance, 39(3), 65-71. https://doi.org/10.1016/j.ssnmr.2011.02.001
Kobayashi, Takeshi, et al. "Molecular ordering of mixed surfactants in mesoporous silicas: a solid-state NMR study." Solid state nuclear magnetic resonance vol. 39,3 (2011): 65-71. doi: https://doi.org/10.1016/j.ssnmr.2011.02.001
Kobayashi T, Mao K, Wang SG, Lin VS, Pruski M. Molecular ordering of mixed surfactants in mesoporous silicas: a solid-state NMR study. Solid State Nucl Magn Reson. 2011 May-Jun;39(3):65-71. doi: 10.1016/j.ssnmr.2011.02.001. Epub 2011 Feb 17. PMID: 21392947.
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Controlling reactivity of nanoporous catalyst materials by tuning reaction product-pore interior interactions: statistical mechanical modeling.

The Journal of chemical physics

Wang J, Ackerman DM, Lin VS, Pruski M, Evans JW.
PMID: 23574250
J Chem Phys. 2013 Apr 07;138(13):134705. doi: 10.1063/1.4798463.

Statistical mechanical modeling is performed of a catalytic conversion reaction within a functionalized nanoporous material to assess the effect of varying the reaction product-pore interior interaction from attractive to repulsive. A strong enhancement in reactivity is observed not just...

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Wang J, Ackerman DM, Lin VS, et al. Controlling reactivity of nanoporous catalyst materials by tuning reaction product-pore interior interactions: statistical mechanical modeling. J Chem Phys. 2013;138(13):134705doi: 10.1063/1.4798463.
Wang, J., Ackerman, D. M., Lin, V. S., Pruski, M., & Evans, J. W. (2013). Controlling reactivity of nanoporous catalyst materials by tuning reaction product-pore interior interactions: statistical mechanical modeling. The Journal of chemical physics, 138(13), 134705. https://doi.org/10.1063/1.4798463
Wang, Jing, et al. "Controlling reactivity of nanoporous catalyst materials by tuning reaction product-pore interior interactions: statistical mechanical modeling." The Journal of chemical physics vol. 138,13 (2013): 134705. doi: https://doi.org/10.1063/1.4798463
Wang J, Ackerman DM, Lin VS, Pruski M, Evans JW. Controlling reactivity of nanoporous catalyst materials by tuning reaction product-pore interior interactions: statistical mechanical modeling. J Chem Phys. 2013 Apr 07;138(13):134705. doi: 10.1063/1.4798463. PMID: 23574250.
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Showing 1 to 12 of 225 entries