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Mechanisms of Heterogeneous Oxidations at Model Aerosol Interfaces by Ozone and Hydroxyl Radicals

EPSCoR Research Infrastructure Improvement Program: Bridging EPSCoR Communities AND Program Evaluation

Pillar-Little EA.
GSID: ei0qMAP6q-wJ
EA Pillar-Little - 2017 - uknowledge.uky.edu

Atmospheric aerosols play an important role in climate by scattering and absorbing radiation and by serving as cloud condensation nuclei. An aerosol's optical or nucleation properties are driven by its chemical composition. Chemical aging of aerosols by atmospheric oxidants,...

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Pillar-Little, E. A. (2017). Mechanisms of Heterogeneous Oxidations at Model Aerosol Interfaces by Ozone and Hydroxyl Radicals.
Pillar-Little, Elizabeth A. "Mechanisms of Heterogeneous Oxidations at Model Aerosol Interfaces by Ozone and Hydroxyl Radicals." (2017).
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Anti-Inflammatory and Anti-Oxidative Nutrition in Hypoalbuminemic Dialysis Patients (AIONID) study: results of the pilot-feasibility, double-blind, randomized, placebo-controlled trial.

Journal of cachexia, sarcopenia and muscle

Rattanasompattikul M, Molnar MZ, Lee ML, Dukkipati R, Bross R, Jing J, Kim Y, Voss AC, Benner D, Feroze U, Macdougall IC, Tayek JA, Norris KC, Kopple JD, Unruh M, Kovesdy CP, Kalantar-Zadeh K.
PMID: 24052226
J Cachexia Sarcopenia Muscle. 2013 Dec;4(4):247-57. doi: 10.1007/s13539-013-0115-9. Epub 2013 Sep 20.

BACKGROUND: Low serum albumin is common and associated with protein-energy wasting, inflammation, and poor outcomes in maintenance hemodialysis (MHD) patients. We hypothesized that in-center (in dialysis clinic) provision of high-protein oral nutrition supplements (ONS) tailored for MHD patients combined...

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Rattanasompattikul M, Molnar MZ, Lee ML, et al. Anti-Inflammatory and Anti-Oxidative Nutrition in Hypoalbuminemic Dialysis Patients (AIONID) study: results of the pilot-feasibility, double-blind, randomized, placebo-controlled trial. J Cachexia Sarcopenia Muscle. 2013;4(4):247-57doi: 10.1007/s13539-013-0115-9.
Rattanasompattikul, M., Molnar, M. Z., Lee, M. L., Dukkipati, R., Bross, R., Jing, J., Kim, Y., Voss, A. C., Benner, D., Feroze, U., Macdougall, I. C., Tayek, J. A., Norris, K. C., Kopple, J. D., Unruh, M., Kovesdy, C. P., & Kalantar-Zadeh, K. (2013). Anti-Inflammatory and Anti-Oxidative Nutrition in Hypoalbuminemic Dialysis Patients (AIONID) study: results of the pilot-feasibility, double-blind, randomized, placebo-controlled trial. Journal of cachexia, sarcopenia and muscle, 4(4), 247-57. https://doi.org/10.1007/s13539-013-0115-9
Rattanasompattikul, Manoch, et al. "Anti-Inflammatory and Anti-Oxidative Nutrition in Hypoalbuminemic Dialysis Patients (AIONID) study: results of the pilot-feasibility, double-blind, randomized, placebo-controlled trial." Journal of cachexia, sarcopenia and muscle vol. 4,4 (2013): 247-57. doi: https://doi.org/10.1007/s13539-013-0115-9
Rattanasompattikul M, Molnar MZ, Lee ML, Dukkipati R, Bross R, Jing J, Kim Y, Voss AC, Benner D, Feroze U, Macdougall IC, Tayek JA, Norris KC, Kopple JD, Unruh M, Kovesdy CP, Kalantar-Zadeh K. Anti-Inflammatory and Anti-Oxidative Nutrition in Hypoalbuminemic Dialysis Patients (AIONID) study: results of the pilot-feasibility, double-blind, randomized, placebo-controlled trial. J Cachexia Sarcopenia Muscle. 2013 Dec;4(4):247-57. doi: 10.1007/s13539-013-0115-9. Epub 2013 Sep 20. PMID: 24052226; PMCID: PMC3830006.
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AOPPs and the progression of kidney disease.

Kidney international supplements

Cao W, Hou FF, Nie J.
PMID: 26312159
Kidney Int Suppl (2011). 2014 Nov;4(1):102-106. doi: 10.1038/kisup.2014.19.

Advanced oxidation protein products (AOPPs) are the dityrosine-containing and crosslinking protein products formed during oxidative stress by reaction of plasma protein with chlorinated oxidants, and often carried by albumin

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Cao W, Hou FF, Nie J. AOPPs and the progression of kidney disease. Kidney Int Suppl (2011). 2014;4(1):102-106doi: 10.1038/kisup.2014.19.
Cao, W., Hou, F. F., & Nie, J. (2014). AOPPs and the progression of kidney disease. Kidney international supplements, 4(1), 102-106. https://doi.org/10.1038/kisup.2014.19
Cao, Wei, et al. "AOPPs and the progression of kidney disease." Kidney international supplements vol. 4,1 (2014): 102-106. doi: https://doi.org/10.1038/kisup.2014.19
Cao W, Hou FF, Nie J. AOPPs and the progression of kidney disease. Kidney Int Suppl (2011). 2014 Nov;4(1):102-106. doi: 10.1038/kisup.2014.19. PMID: 26312159; PMCID: PMC4536974.
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Acid- and Au(i)-mediated synthesis of hexathymidine-DNA-heterocycle chimeras, an efficient entry to DNA-encoded libraries inspired by drug structures.

Chemical science

Škopić MK, Salamon H, Bugain O, Jung K, Gohla A, Doetsch LJ, Dos Santos D, Bhat A, Wagner B, Brunschweiger A.
PMID: 28507705
Chem Sci. 2017 May 01;8(5):3356-3361. doi: 10.1039/c7sc00455a. Epub 2017 Feb 28.

Libraries of DNA-tagged compounds are a validated screening technology for drug discovery. They are synthesized through combinatorial iterations of alternated coding and preparative synthesis steps. Thus, large chemical space can be accessed for target-based screening. However, the need to...

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Škopić MK, Salamon H, Bugain O, et al. Acid- and Au(i)-mediated synthesis of hexathymidine-DNA-heterocycle chimeras, an efficient entry to DNA-encoded libraries inspired by drug structures. Chem Sci. 2017;8(5):3356-3361doi: 10.1039/c7sc00455a.
Škopić, M. K., Salamon, H., Bugain, O., Jung, K., Gohla, A., Doetsch, L. J., Dos Santos, D., Bhat, A., Wagner, B., & Brunschweiger, A. (2017). Acid- and Au(i)-mediated synthesis of hexathymidine-DNA-heterocycle chimeras, an efficient entry to DNA-encoded libraries inspired by drug structures. Chemical science, 8(5), 3356-3361. https://doi.org/10.1039/c7sc00455a
Škopić, Mateja Klika, et al. "Acid- and Au(i)-mediated synthesis of hexathymidine-DNA-heterocycle chimeras, an efficient entry to DNA-encoded libraries inspired by drug structures." Chemical science vol. 8,5 (2017): 3356-3361. doi: https://doi.org/10.1039/c7sc00455a
Škopić MK, Salamon H, Bugain O, Jung K, Gohla A, Doetsch LJ, Dos Santos D, Bhat A, Wagner B, Brunschweiger A. Acid- and Au(i)-mediated synthesis of hexathymidine-DNA-heterocycle chimeras, an efficient entry to DNA-encoded libraries inspired by drug structures. Chem Sci. 2017 May 01;8(5):3356-3361. doi: 10.1039/c7sc00455a. Epub 2017 Feb 28. PMID: 28507705; PMCID: PMC5416911.
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Theoretical Investigation of Anion-Radical States of Edge-Oxidized Carbon Model Clusters.

The journal of physical chemistry. A

Khavryuchenko OV, Frank B.
PMID: 28391687
J Phys Chem A. 2017 Apr 27;121(16):3167-3173. doi: 10.1021/acs.jpca.7b02437. Epub 2017 Apr 14.

A set of flat carbon clusters and ultrashort carbon nanotubes in different anion-radical states was investigated by density functional theory and complete-active space self-consistent field methods. It was found that carbon nanoparticles with pervasively oxidized edges are extremely strong...

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Khavryuchenko OV, Frank B. Theoretical Investigation of Anion-Radical States of Edge-Oxidized Carbon Model Clusters. J Phys Chem A. 2017;121(16):3167-3173doi: 10.1021/acs.jpca.7b02437.
Khavryuchenko, O. V., & Frank, B. (2017). Theoretical Investigation of Anion-Radical States of Edge-Oxidized Carbon Model Clusters. The journal of physical chemistry. A, 121(16), 3167-3173. https://doi.org/10.1021/acs.jpca.7b02437
Khavryuchenko, Oleksiy V, and Frank, Benjamin. "Theoretical Investigation of Anion-Radical States of Edge-Oxidized Carbon Model Clusters." The journal of physical chemistry. A vol. 121,16 (2017): 3167-3173. doi: https://doi.org/10.1021/acs.jpca.7b02437
Khavryuchenko OV, Frank B. Theoretical Investigation of Anion-Radical States of Edge-Oxidized Carbon Model Clusters. J Phys Chem A. 2017 Apr 27;121(16):3167-3173. doi: 10.1021/acs.jpca.7b02437. Epub 2017 Apr 14. PMID: 28391687.
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Facile formation of homoleptic Au(III) trications via simultaneous oxidation and ligand delivery from [PhI(pyridine)2](2+).

Journal of the American Chemical Society

Corbo R, Pell TP, Stringer BD, Hogan CF, Wilson DJ, Barnard PJ, Dutton JL.
PMID: 25116433
J Am Chem Soc. 2014 Sep 03;136(35):12415-21. doi: 10.1021/ja506365m. Epub 2014 Aug 21.

We report the first examples of Au(III) tricationic complexes bound only by neutral monodentate ligands, which are a new class of gold reagents. Oxidative addition to the bis-pyridine Au(I) cation, [Au(4-DMAP)2](+), using a series of dicationic I(III) oxidants of...

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Corbo R, Pell TP, Stringer BD, et al. Facile formation of homoleptic Au(III) trications via simultaneous oxidation and ligand delivery from [PhI(pyridine)2](2+). J Am Chem Soc. 2014;136(35):12415-21doi: 10.1021/ja506365m.
Corbo, R., Pell, T. P., Stringer, B. D., Hogan, C. F., Wilson, D. J., Barnard, P. J., & Dutton, J. L. (2014). Facile formation of homoleptic Au(III) trications via simultaneous oxidation and ligand delivery from [PhI(pyridine)2](2+). Journal of the American Chemical Society, 136(35), 12415-21. https://doi.org/10.1021/ja506365m
Corbo, Robert, et al. "Facile formation of homoleptic Au(III) trications via simultaneous oxidation and ligand delivery from [PhI(pyridine)2](2+)." Journal of the American Chemical Society vol. 136,35 (2014): 12415-21. doi: https://doi.org/10.1021/ja506365m
Corbo R, Pell TP, Stringer BD, Hogan CF, Wilson DJ, Barnard PJ, Dutton JL. Facile formation of homoleptic Au(III) trications via simultaneous oxidation and ligand delivery from [PhI(pyridine)2](2+). J Am Chem Soc. 2014 Sep 03;136(35):12415-21. doi: 10.1021/ja506365m. Epub 2014 Aug 21. PMID: 25116433.
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O-Acyl oximes: versatile building blocks for N-heterocycle formation in recent transition metal catalysis.

Organic & biomolecular chemistry

Huang H, Cai J, Deng GJ.
PMID: 26727109
Org Biomol Chem. 2016 Feb 07;14(5):1519-30. doi: 10.1039/c5ob02417j.

O-Acyl oximes are versatile building blocks being widely applied in organic synthesis, especially for N-heterocycle construction under transition metal catalysis. In the last decade, aza-Heck cyclization using oximes has been progressing in the preparation of functionalized pyrrolines, and instead...

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Huang H, Cai J, Deng GJ. O-Acyl oximes: versatile building blocks for N-heterocycle formation in recent transition metal catalysis. Org Biomol Chem. 2016;14(5):1519-30doi: 10.1039/c5ob02417j.
Huang, H., Cai, J., & Deng, G. J. (2016). O-Acyl oximes: versatile building blocks for N-heterocycle formation in recent transition metal catalysis. Organic & biomolecular chemistry, 14(5), 1519-30. https://doi.org/10.1039/c5ob02417j
Huang, Huawen, et al. "O-Acyl oximes: versatile building blocks for N-heterocycle formation in recent transition metal catalysis." Organic & biomolecular chemistry vol. 14,5 (2016): 1519-30. doi: https://doi.org/10.1039/c5ob02417j
Huang H, Cai J, Deng GJ. O-Acyl oximes: versatile building blocks for N-heterocycle formation in recent transition metal catalysis. Org Biomol Chem. 2016 Feb 07;14(5):1519-30. doi: 10.1039/c5ob02417j. PMID: 26727109.
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Data on how several physiological parameters of stored red blood cells are similar in glucose 6-phosphate dehydrogenase deficient and sufficient donors.

Data in brief

Tzounakas VL, Kriebardis AG, Georgatzakou HT, Foudoulaki-Paparizos LE, Dzieciatkowska M, Wither MJ, Nemkov T, Hansen KC, Papassideri IS, D'Alessandro A, Antonelou MH.
PMID: 27437434
Data Brief. 2016 Jun 23;8:618-27. doi: 10.1016/j.dib.2016.06.018. eCollection 2016 Sep.

This article contains data on the variation in several physiological parameters of red blood cells (RBCs) donated by eligible glucose-6-phosphate dehydrogenase (G6PD) deficient donors during storage in standard blood bank conditions compared to control, G6PD sufficient (G6PD(+)) cells. Intracellular...

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Tzounakas VL, Kriebardis AG, Georgatzakou HT, et al. Data on how several physiological parameters of stored red blood cells are similar in glucose 6-phosphate dehydrogenase deficient and sufficient donors. Data Brief. 2016;8:618-27doi: 10.1016/j.dib.2016.06.018.
Tzounakas, V. L., Kriebardis, A. G., Georgatzakou, H. T., Foudoulaki-Paparizos, L. E., Dzieciatkowska, M., Wither, M. J., Nemkov, T., Hansen, K. C., Papassideri, I. S., D'Alessandro, A., & Antonelou, M. H. (2016). Data on how several physiological parameters of stored red blood cells are similar in glucose 6-phosphate dehydrogenase deficient and sufficient donors. Data in brief, 8618-27. https://doi.org/10.1016/j.dib.2016.06.018
Tzounakas, Vassilis L, et al. "Data on how several physiological parameters of stored red blood cells are similar in glucose 6-phosphate dehydrogenase deficient and sufficient donors." Data in brief vol. 8 (2016): 618-27. doi: https://doi.org/10.1016/j.dib.2016.06.018
Tzounakas VL, Kriebardis AG, Georgatzakou HT, Foudoulaki-Paparizos LE, Dzieciatkowska M, Wither MJ, Nemkov T, Hansen KC, Papassideri IS, D'Alessandro A, Antonelou MH. Data on how several physiological parameters of stored red blood cells are similar in glucose 6-phosphate dehydrogenase deficient and sufficient donors. Data Brief. 2016 Jun 23;8:618-27. doi: 10.1016/j.dib.2016.06.018. eCollection 2016 Sep. PMID: 27437434; PMCID: PMC4939423.
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Oxidative Stress and the Use of Antioxidants in Stroke.

Antioxidants (Basel, Switzerland)

Shirley R, Ord EN, Work LM.
PMID: 26785066
Antioxidants (Basel). 2014 Jul 03;3(3):472-501. doi: 10.3390/antiox3030472.

Transient or permanent interruption of cerebral blood flow by occlusion of a cerebral artery gives rise to an ischaemic stroke leading to irreversible damage or dysfunction to the cells within the affected tissue along with permanent or reversible neurological...

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Shirley R, Ord EN, Work LM. Oxidative Stress and the Use of Antioxidants in Stroke. Antioxidants (Basel). 2014;3(3):472-501doi: 10.3390/antiox3030472.
Shirley, R., Ord, E. N., & Work, L. M. (2014). Oxidative Stress and the Use of Antioxidants in Stroke. Antioxidants (Basel, Switzerland), 3(3), 472-501. https://doi.org/10.3390/antiox3030472
Shirley, Rachel, et al. "Oxidative Stress and the Use of Antioxidants in Stroke." Antioxidants (Basel, Switzerland) vol. 3,3 (2014): 472-501. doi: https://doi.org/10.3390/antiox3030472
Shirley R, Ord EN, Work LM. Oxidative Stress and the Use of Antioxidants in Stroke. Antioxidants (Basel). 2014 Jul 03;3(3):472-501. doi: 10.3390/antiox3030472. PMID: 26785066; PMCID: PMC4665418.
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Geological and Geochemical Controls on Subsurface Microbial Life in the Samail Ophiolite, Oman.

Frontiers in microbiology

Rempfert KR, Miller HM, Bompard N, Nothaft D, Matter JM, Kelemen P, Fierer N, Templeton AS.
PMID: 28223966
Front Microbiol. 2017 Feb 07;8:56. doi: 10.3389/fmicb.2017.00056. eCollection 2017.

Microbial abundance and diversity in deep subsurface environments is dependent upon the availability of energy and carbon. However, supplies of oxidants and reductants capable of sustaining life within mafic and ultramafic continental aquifers undergoing low-temperature water-rock reaction are relatively...

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Rempfert KR, Miller HM, Bompard N, et al. Geological and Geochemical Controls on Subsurface Microbial Life in the Samail Ophiolite, Oman. Front Microbiol. 2017;8:56doi: 10.3389/fmicb.2017.00056.
Rempfert, K. R., Miller, H. M., Bompard, N., Nothaft, D., Matter, J. M., Kelemen, P., Fierer, N., & Templeton, A. S. (2017). Geological and Geochemical Controls on Subsurface Microbial Life in the Samail Ophiolite, Oman. Frontiers in microbiology, 856. https://doi.org/10.3389/fmicb.2017.00056
Rempfert, Kaitlin R, et al. "Geological and Geochemical Controls on Subsurface Microbial Life in the Samail Ophiolite, Oman." Frontiers in microbiology vol. 8 (2017): 56. doi: https://doi.org/10.3389/fmicb.2017.00056
Rempfert KR, Miller HM, Bompard N, Nothaft D, Matter JM, Kelemen P, Fierer N, Templeton AS. Geological and Geochemical Controls on Subsurface Microbial Life in the Samail Ophiolite, Oman. Front Microbiol. 2017 Feb 07;8:56. doi: 10.3389/fmicb.2017.00056. eCollection 2017. PMID: 28223966; PMCID: PMC5293757.
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Beyond the Dimer and Trimer: Tetraspiro[2.1.2(5).1.2(9).1.2(13).1(3)] hexadecane-1,3,5,7-tetraone--the Cyclic Tetramer of Carbonylcyclopropane.

Chemistry (Weinheim an der Bergstrasse, Germany)

Sedenkova KN, Averina EB, Grishin YK, Andriasov KS, Stepanova SA, Roznyatovsky VA, Kutateladze AG, Rybakov VB, Albov DV, Kuznetsova TS, Zefirov NS.
PMID: 26762227
Chemistry. 2016 Mar 14;22(12):3996-9. doi: 10.1002/chem.201600140. Epub 2016 Feb 03.

Tetraspiro[2.1.2(5).1.2(9).1.2(13).1(3)]hexadecane-1,3,5,7-tetraone 4, a unique tetraketone containing a cyclooctane core and four spiroannelated cyclopropane moieties, represents the previously unknown cyclotetramer of carbonylcyclopropane. For this purpose oxidation of the parent polyspirocyclic hydrocarbon was examined under various oxidative conditions, and the reactivity...

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Sedenkova KN, Averina EB, Grishin YK, et al. Beyond the Dimer and Trimer: Tetraspiro[2.1.2(5).1.2(9).1.2(13).1(3)] hexadecane-1,3,5,7-tetraone--the Cyclic Tetramer of Carbonylcyclopropane. Chemistry. 2016;22(12):3996-9doi: 10.1002/chem.201600140.
Sedenkova, K. N., Averina, E. B., Grishin, Y. K., Andriasov, K. S., Stepanova, S. A., Roznyatovsky, V. A., Kutateladze, A. G., Rybakov, V. B., Albov, D. V., Kuznetsova, T. S., & Zefirov, N. S. (2016). Beyond the Dimer and Trimer: Tetraspiro[2.1.2(5).1.2(9).1.2(13).1(3)] hexadecane-1,3,5,7-tetraone--the Cyclic Tetramer of Carbonylcyclopropane. Chemistry (Weinheim an der Bergstrasse, Germany), 22(12), 3996-9. https://doi.org/10.1002/chem.201600140
Sedenkova, Kseniya N, et al. "Beyond the Dimer and Trimer: Tetraspiro[2.1.2(5).1.2(9).1.2(13).1(3)] hexadecane-1,3,5,7-tetraone--the Cyclic Tetramer of Carbonylcyclopropane." Chemistry (Weinheim an der Bergstrasse, Germany) vol. 22,12 (2016): 3996-9. doi: https://doi.org/10.1002/chem.201600140
Sedenkova KN, Averina EB, Grishin YK, Andriasov KS, Stepanova SA, Roznyatovsky VA, Kutateladze AG, Rybakov VB, Albov DV, Kuznetsova TS, Zefirov NS. Beyond the Dimer and Trimer: Tetraspiro[2.1.2(5).1.2(9).1.2(13).1(3)] hexadecane-1,3,5,7-tetraone--the Cyclic Tetramer of Carbonylcyclopropane. Chemistry. 2016 Mar 14;22(12):3996-9. doi: 10.1002/chem.201600140. Epub 2016 Feb 03. PMID: 26762227.
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Regioselective oxidative Pd-catalysed coupling of alkylboronic acids with pyridin-2-yl-substituted heterocycles.

Chemical communications (Cambridge, England)

Wippich J, Schnapperelle I, Bach T.
PMID: 25605647
Chem Commun (Camb). 2015 Feb 21;51(15):3166-8. doi: 10.1039/c4cc10144h.

A total of 19 alkylated heterocycles (thiophenes, benzothiophenes, pyrroles, furans) were prepared (36-99% yield) from the respective pyridin-2-yl-substituted precursors employing alkylboronic acids as the C-H alkylating reagents in an oxidative (Ag2CO3 and 2,6-dimethyl-1,4-benzoquinone as oxidants) Pd-catalysed coupling reaction.

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Wippich J, Schnapperelle I, Bach T. Regioselective oxidative Pd-catalysed coupling of alkylboronic acids with pyridin-2-yl-substituted heterocycles. Chem Commun (Camb). 2015;51(15):3166-8doi: 10.1039/c4cc10144h.
Wippich, J., Schnapperelle, I., & Bach, T. (2015). Regioselective oxidative Pd-catalysed coupling of alkylboronic acids with pyridin-2-yl-substituted heterocycles. Chemical communications (Cambridge, England), 51(15), 3166-8. https://doi.org/10.1039/c4cc10144h
Wippich, Julian, et al. "Regioselective oxidative Pd-catalysed coupling of alkylboronic acids with pyridin-2-yl-substituted heterocycles." Chemical communications (Cambridge, England) vol. 51,15 (2015): 3166-8. doi: https://doi.org/10.1039/c4cc10144h
Wippich J, Schnapperelle I, Bach T. Regioselective oxidative Pd-catalysed coupling of alkylboronic acids with pyridin-2-yl-substituted heterocycles. Chem Commun (Camb). 2015 Feb 21;51(15):3166-8. doi: 10.1039/c4cc10144h. PMID: 25605647.
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