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Morimoto K, Ohnishi Y, Koseki D, et al. Stabilized pyrrolyl iodonium salts and metal-free oxidative cross-coupling. Org Biomol Chem. 2016;14(38):8947-8951doi: 10.1039/c6ob01764a.
Morimoto, K., Ohnishi, Y., Koseki, D., Nakamura, A., Dohi, T., & Kita, Y. (2016). Stabilized pyrrolyl iodonium salts and metal-free oxidative cross-coupling. Organic & biomolecular chemistry, 14(38), 8947-8951. https://doi.org/10.1039/c6ob01764a
Morimoto, Koji, et al. "Stabilized pyrrolyl iodonium salts and metal-free oxidative cross-coupling." Organic & biomolecular chemistry vol. 14,38 (2016): 8947-8951. doi: https://doi.org/10.1039/c6ob01764a
Morimoto K, Ohnishi Y, Koseki D, Nakamura A, Dohi T, Kita Y. Stabilized pyrrolyl iodonium salts and metal-free oxidative cross-coupling. Org Biomol Chem. 2016 Sep 26;14(38):8947-8951. doi: 10.1039/c6ob01764a. PMID: 27722732.
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Org Biomol Chem. 2016 Sep 26;14(38):8947-8951. doi: 10.1039/c6ob01764a.

Stabilized pyrrolyl iodonium salts and metal-free oxidative cross-coupling.

Organic & biomolecular chemistry

Koji Morimoto, Yusuke Ohnishi, Daichi Koseki, Akira Nakamura, Toshifumi Dohi, Yasuyuki Kita

Affiliations

  1. Ritsumeikan University, College of Pharmaceutical Sciences, 1-1-1 Nojihigashi, Kusatsu, Shiga 525-8577, Japan.
  2. Ritsumeikan University, Research Organization of Science and Technology, 1-1-1 Nojihigashi, Kusatsu, Shiga 525-8577, Japan. [email protected].

PMID: 27722732 DOI: 10.1039/c6ob01764a

Abstract

Pyrrole-aryl derivatives are important due to their unique biological activities in medicinal chemistry. We now report a new oxidative biaryl coupling for pyrroles and indoles toward various arenes using a hypervalent iodine reagent and an appropriate stabilizer for pyrrolyl iodonium intermediates. The reactions readily provide a variety of desired coupling products in good yields.

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